Room-temperature continuous-wave pumped exciton polariton condensation in a perovskite microcavity

被引:3
作者
Song, Jiepeng [1 ]
Ghosh, Sanjib [2 ]
Deng, Xinyi [1 ]
Li, Chun [1 ]
Shang, Qiuyu [1 ]
Liu, Xinfeng [3 ]
Wang, Yubin [4 ,5 ]
Gao, Xiaoyue [6 ]
Yang, Wenkai [6 ]
Wang, Xianjin [6 ]
Zhao, Qing [6 ]
Shi, Kebin [6 ]
Gao, Peng [6 ]
Xing, Guichuan [7 ]
Xiong, Qihua [2 ,4 ,5 ]
Zhang, Qing [1 ]
机构
[1] Peking Univ, Sch Mat Sci & Engn, Beijing 100871, Peoples R China
[2] Beijing Acad Quantum Informat Sci, Beijing 100094, Peoples R China
[3] Natl Ctr Nanosci & Technol, CAS Key Lab Standardizat & Measurement Nanotechnol, Beijing 100190, Peoples R China
[4] Tsinghua Univ, State Key Lab Low Dimens Quantum Phys, Beijing 100084, Peoples R China
[5] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China
[6] Peking Univ, Sch Phys, Beijing 100871, Peoples R China
[7] Univ Macao, Inst Joint Key Lab Appl Phys & Mat Engn, Taipa 999078, Macau, Peoples R China
基金
美国国家科学基金会; 北京市自然科学基金; 中国国家自然科学基金;
关键词
BOSE-EINSTEIN CONDENSATION;
D O I
10.1126/sciadv.adr1652
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Microcavity exciton polaritons (polaritons) as part-light part-matter quasiparticles garner considerable attention for Bose-Einstein condensation at elevated temperatures. Recently, halide perovskites have emerged as promising room-temperature polaritonic platforms because of their large exciton binding energies and superior optical properties. However, currently, inducing room-temperature nonequilibrium polariton condensation in perovskite microcavities requires optical pulsed excitations with high excitation densities. Here, we demonstrate continuous-wave optically pumped polariton condensation with an exceptionally low threshold of similar to 0.53 W cm(-2) and a narrow linewidth of similar to 0.5 meV. Polariton condensation is unambiguously demonstrated by characterizing the nonlinear behavior and coherence properties. We also unveil the trapping potential landscape strategy to facilitate polariton relaxation and accumulation. Our findings lay the foundation for the next-generation energy-efficient polaritonic devices operating at room temperature.
引用
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页数:10
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