Environmental barrier coating;
High entropy rare earth pyrosilicate;
Water vapor corrosion;
Binding energy;
D O I:
10.1016/j.surfcoat.2025.131907
中图分类号:
TB3 [工程材料学];
学科分类号:
0805 ;
080502 ;
摘要:
Improving water vapor corrosion resistance has become critical for environmental barrier coating materials to extend the life of ceramic matrix composites. A novel environmental barrier coating candidate (Yb0.2Y0.2Lu0.2Er0.2Sc0.2)2Si2O7((5RE1/5)2Si2O7) was synthesized in this study. The corrosion behavior of (5RE1/5)2Si2O7 in a water vapor environment at 1400 degrees C was observed and analyzed. The results show that (5RE1/5)2Si2O7 is a high-performance environmental barrier coating material against water vapor corrosion. Corrosion pores and transcrystalline cracks appeared on the surface of the material after 300 h of corrosion. The average thickness of the recession layer was about 5.66 mu m. The pyrosilicate phase still occupied 87.834 %. The mass loss rate of the material was about 0.0396 mg/cm2. The corrosion resistance is superior to the disclosed coating materials. This research provided a theoretical basis for optimizing the performance of environmental barrier coatings.
机构:
Wuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R ChinaWuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R China
Luo, Zhongwei
Jiang, Jianing
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机构:
Wuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R ChinaWuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R China
Jiang, Jianing
Dong, Shujuan
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机构:
Wuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R ChinaWuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R China
Dong, Shujuan
Zhou, Changling
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机构:
Shandong Ind Ceram Res & Design Inst, Zibo 255000, Peoples R ChinaWuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R China
Zhou, Changling
Lue, Kaiyue
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机构:
Wuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R ChinaWuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R China
Lue, Kaiyue
Xie, Yifeng
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Wuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R ChinaWuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R China
Xie, Yifeng
Duan, Zhixing
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机构:
Wuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R ChinaWuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R China
Duan, Zhixing
Huang, Yan
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机构:
Wuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R ChinaWuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R China
Huang, Yan
Chen, Tingyang
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Wuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R ChinaWuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R China
Chen, Tingyang
Deng, Longhui
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机构:
Wuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R ChinaWuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R China
Deng, Longhui
Cao, Xueqiang
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机构:
Wuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R ChinaWuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R China
机构:
School of Materials Science and Engineering, Harbin Institute of Technology, Harbin,150001, ChinaSchool of Materials Science and Engineering, Harbin Institute of Technology, Harbin,150001, China
Wei, Fushuang
Deng, Luwei
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机构:
School of Materials Science and Engineering, Harbin Institute of Technology, Harbin,150001, ChinaSchool of Materials Science and Engineering, Harbin Institute of Technology, Harbin,150001, China
Deng, Luwei
Liu, Yong
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机构:
School of Materials Science and Engineering, Harbin Institute of Technology, Harbin,150001, ChinaSchool of Materials Science and Engineering, Harbin Institute of Technology, Harbin,150001, China
Liu, Yong
Zhang, Dongxing
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机构:
School of Materials Science and Engineering, Harbin Institute of Technology, Harbin,150001, ChinaSchool of Materials Science and Engineering, Harbin Institute of Technology, Harbin,150001, China
Zhang, Dongxing
Zhang, Xiaodong
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机构:
School of Materials Science and Engineering, Harbin Institute of Technology, Harbin,150001, ChinaSchool of Materials Science and Engineering, Harbin Institute of Technology, Harbin,150001, China
Zhang, Xiaodong
Wang, You
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h-index: 0
机构:
School of Materials Science and Engineering, Harbin Institute of Technology, Harbin,150001, ChinaSchool of Materials Science and Engineering, Harbin Institute of Technology, Harbin,150001, China
机构:
Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine M, Shanghai 200050, Peoples R China
Univ Chinese Acad Sci, Ctr Mat Sci & Optoelect Engn, Beijing 100049, Peoples R ChinaChinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine M, Shanghai 200050, Peoples R China
Chen, Zeyu
Lin, Chucheng
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h-index: 0
机构:
Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine M, Shanghai 200050, Peoples R ChinaChinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine M, Shanghai 200050, Peoples R China
Lin, Chucheng
Zheng, Wei
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h-index: 0
机构:
Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine M, Shanghai 200050, Peoples R ChinaChinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine M, Shanghai 200050, Peoples R China
Zheng, Wei
Jiang, Caifen
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h-index: 0
机构:
Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine M, Shanghai 200050, Peoples R ChinaChinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine M, Shanghai 200050, Peoples R China
Jiang, Caifen
Song, Xuemei
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine M, Shanghai 200050, Peoples R China
Univ Chinese Acad Sci, Ctr Mat Sci & Optoelect Engn, Beijing 100049, Peoples R ChinaChinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine M, Shanghai 200050, Peoples R China
Song, Xuemei
Zeng, Yi
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h-index: 0
机构:
Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine M, Shanghai 200050, Peoples R China
Shanghai Inst Ceram, 585 Heshuo Rd, Shanghai, Peoples R ChinaChinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine M, Shanghai 200050, Peoples R China
机构:
Science and Technology on Thermostructural Composite Materials Laboratory, Northwestern Polytechnical UniversityScience and Technology on Thermostructural Composite Materials Laboratory, Northwestern Polytechnical University
Yu DONG
Ke REN
论文数: 0引用数: 0
h-index: 0
机构:
Institute of Advanced Structure Technology, Beijing Institute of TechnologyScience and Technology on Thermostructural Composite Materials Laboratory, Northwestern Polytechnical University
Ke REN
Qiankun WANG
论文数: 0引用数: 0
h-index: 0
机构:
Science and Technology on Thermostructural Composite Materials Laboratory, Northwestern Polytechnical UniversityScience and Technology on Thermostructural Composite Materials Laboratory, Northwestern Polytechnical University
Qiankun WANG
Gang SHAO
论文数: 0引用数: 0
h-index: 0
机构:
Henan Province Industrial Technology Research Institute of Resources and Materials, Zhengzhou UniversityScience and Technology on Thermostructural Composite Materials Laboratory, Northwestern Polytechnical University
Gang SHAO
Yiguang WANG
论文数: 0引用数: 0
h-index: 0
机构:
Institute of Advanced Structure Technology, Beijing Institute of TechnologyScience and Technology on Thermostructural Composite Materials Laboratory, Northwestern Polytechnical University