Two alternative coal-to-aromatics processes, the methane steam reforming-assisted process (NG-CTA-S) and methane dry/steam reforming-integrated process (NG-CTA-DS), are proposed to mitigate carbon dioxide (CO2) emissions associated with conventional coal-to-aromatics (CTA) processes. This study conducted a detailed process simulation and optimization of key parameters to determine the aromatic production route with the lowest carbon emission. A comprehensive technical and economic analysis, along with an environmental assessment, was carried out to compare the proposed processes with existing ones. The results indicate that the NG-CTA-DS process has demonstrated superior techno-economic performance and environmental evaluation. It achieved an elemental carbon utilization of 85.95 %, an energy efficiency of 78.80 %, a reduced CO2 emission of 3.65 kg/kg-aromatics, and a production cost of only 1018.87 M$. Therefore, it is evident that the proposed NGCTA-DS process holds significant potential to enhance the technical, economic, and environmental performance compared to the conventional process, making it a promising candidate for industrialization.
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Univ Sao Paulo, Dept Chem Engn, Escola Politecn, Ave Prof Luciano Gualberto,380, BR-05508010 Sao Paulo, SP, BrazilUniv Sao Paulo, Dept Chem Engn, Escola Politecn, Ave Prof Luciano Gualberto,380, BR-05508010 Sao Paulo, SP, Brazil
Santos, Magno Fonseca
Bresciani, Antonio Esio
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Univ Sao Paulo, Dept Chem Engn, Escola Politecn, Ave Prof Luciano Gualberto,380, BR-05508010 Sao Paulo, SP, BrazilUniv Sao Paulo, Dept Chem Engn, Escola Politecn, Ave Prof Luciano Gualberto,380, BR-05508010 Sao Paulo, SP, Brazil
Bresciani, Antonio Esio
Teixeira, Alexandre Mendonca
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Repsol Sinopec Brasil, Praia Botafogo,300, BR-22250040 Rio de Janeiro, RJ, BrazilUniv Sao Paulo, Dept Chem Engn, Escola Politecn, Ave Prof Luciano Gualberto,380, BR-05508010 Sao Paulo, SP, Brazil
Teixeira, Alexandre Mendonca
Alves, Rita Maria Brito
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Univ Sao Paulo, Dept Chem Engn, Escola Politecn, Ave Prof Luciano Gualberto,380, BR-05508010 Sao Paulo, SP, BrazilUniv Sao Paulo, Dept Chem Engn, Escola Politecn, Ave Prof Luciano Gualberto,380, BR-05508010 Sao Paulo, SP, Brazil
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S China Univ Technol, Sch Chem Engn, Guangzhou 510640, Guangdong, Peoples R ChinaS China Univ Technol, Sch Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
Xiang, Dong
Qian, Yu
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S China Univ Technol, Sch Chem Engn, Guangzhou 510640, Guangdong, Peoples R ChinaS China Univ Technol, Sch Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
Qian, Yu
Man, Yi
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S China Univ Technol, Sch Chem Engn, Guangzhou 510640, Guangdong, Peoples R ChinaS China Univ Technol, Sch Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
Man, Yi
Yang, Siyu
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S China Univ Technol, Sch Chem Engn, Guangzhou 510640, Guangdong, Peoples R ChinaS China Univ Technol, Sch Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
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Lehigh Univ, Dept Mech Engn & Mech, Bethlehem, PA 18015 USA
Lehigh Univ, Energy Res Ctr, 117 ATLSS Dr, Bethlehem, PA 18015 USALehigh Univ, Dept Mech Engn & Mech, Bethlehem, PA 18015 USA
Banerjee, Tanumoy
Bravo, Julio
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Lehigh Univ, Dept Mech Engn & Mech, Bethlehem, PA 18015 USA
Lehigh Univ, Energy Res Ctr, 117 ATLSS Dr, Bethlehem, PA 18015 USA
Lehigh Univ, Inst Cyber Phys Infrastructure & Energy, Bethlehem, PA 18015 USALehigh Univ, Dept Mech Engn & Mech, Bethlehem, PA 18015 USA
Bravo, Julio
Romero, Carlos E.
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Lehigh Univ, Dept Mech Engn & Mech, Bethlehem, PA 18015 USA
Lehigh Univ, Energy Res Ctr, 117 ATLSS Dr, Bethlehem, PA 18015 USA
Lehigh Univ, Inst Cyber Phys Infrastructure & Energy, Bethlehem, PA 18015 USALehigh Univ, Dept Mech Engn & Mech, Bethlehem, PA 18015 USA
Romero, Carlos E.
Lowe, Tom
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Blaschak Anthracite Corp, Mahanoy City, PA 17948 USALehigh Univ, Dept Mech Engn & Mech, Bethlehem, PA 18015 USA
Lowe, Tom
Driscoll, Greg
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Blaschak Anthracite Corp, Mahanoy City, PA 17948 USALehigh Univ, Dept Mech Engn & Mech, Bethlehem, PA 18015 USA
Driscoll, Greg
Kreglow, Boyd
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Blaschak Anthracite Corp, Mahanoy City, PA 17948 USALehigh Univ, Dept Mech Engn & Mech, Bethlehem, PA 18015 USA
Kreglow, Boyd
Schobert, Harold
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Blaschak Anthracite Corp, Mahanoy City, PA 17948 USALehigh Univ, Dept Mech Engn & Mech, Bethlehem, PA 18015 USA
Schobert, Harold
Yao, Zheng
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Lehigh Univ, Energy Res Ctr, 117 ATLSS Dr, Bethlehem, PA 18015 USALehigh Univ, Dept Mech Engn & Mech, Bethlehem, PA 18015 USA