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Coal-to-aromatics process integrated with dry/steam-mixed reforming: Techno-economic analysis and environmental evaluation
被引:0
作者:
Zhang, Junqiang
[1
]
Dong, Peng
[2
]
Lei, Haifeng
[1
]
Liu, Ruonan
[1
]
Wang, Junwen
[1
]
Zhao, Zhitong
[1
]
Zhang, Wei
[1
]
机构:
[1] Taiyuan Univ Technol, Coll Chem Engn & Technol, Taiyuan 030024, Shanxi, Peoples R China
[2] Lanzhou Univ Technol, Sch Petrochem Engn, Lanzhou 730050, Gansu, Peoples R China
基金:
中国国家自然科学基金;
关键词:
Coal-to-aromatics;
CO;
2;
utilization;
Natural gas;
Techno-economic analysis;
Cleaner production;
LIFE-CYCLE ASSESSMENT;
NATURAL-GAS SNG;
ENERGY-CONSUMPTION;
CONCEPTUAL DESIGN;
SYNGAS PRODUCTION;
COMBINED STEAM;
GHG EMISSIONS;
SIMULATION;
METHANOL;
CO2;
D O I:
10.1016/j.ces.2024.120934
中图分类号:
TQ [化学工业];
学科分类号:
0817 ;
摘要:
Two alternative coal-to-aromatics processes, the methane steam reforming-assisted process (NG-CTA-S) and methane dry/steam reforming-integrated process (NG-CTA-DS), are proposed to mitigate carbon dioxide (CO2) emissions associated with conventional coal-to-aromatics (CTA) processes. This study conducted a detailed process simulation and optimization of key parameters to determine the aromatic production route with the lowest carbon emission. A comprehensive technical and economic analysis, along with an environmental assessment, was carried out to compare the proposed processes with existing ones. The results indicate that the NG-CTA-DS process has demonstrated superior techno-economic performance and environmental evaluation. It achieved an elemental carbon utilization of 85.95 %, an energy efficiency of 78.80 %, a reduced CO2 emission of 3.65 kg/kg-aromatics, and a production cost of only 1018.87 M$. Therefore, it is evident that the proposed NGCTA-DS process holds significant potential to enhance the technical, economic, and environmental performance compared to the conventional process, making it a promising candidate for industrialization.
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页数:13
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