Coal-to-aromatics process integrated with dry/steam-mixed reforming: Techno-economic analysis and environmental evaluation

被引:0
作者
Zhang, Junqiang [1 ]
Dong, Peng [2 ]
Lei, Haifeng [1 ]
Liu, Ruonan [1 ]
Wang, Junwen [1 ]
Zhao, Zhitong [1 ]
Zhang, Wei [1 ]
机构
[1] Taiyuan Univ Technol, Coll Chem Engn & Technol, Taiyuan 030024, Shanxi, Peoples R China
[2] Lanzhou Univ Technol, Sch Petrochem Engn, Lanzhou 730050, Gansu, Peoples R China
基金
中国国家自然科学基金;
关键词
Coal-to-aromatics; CO; 2; utilization; Natural gas; Techno-economic analysis; Cleaner production; LIFE-CYCLE ASSESSMENT; NATURAL-GAS SNG; ENERGY-CONSUMPTION; CONCEPTUAL DESIGN; SYNGAS PRODUCTION; COMBINED STEAM; GHG EMISSIONS; SIMULATION; METHANOL; CO2;
D O I
10.1016/j.ces.2024.120934
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Two alternative coal-to-aromatics processes, the methane steam reforming-assisted process (NG-CTA-S) and methane dry/steam reforming-integrated process (NG-CTA-DS), are proposed to mitigate carbon dioxide (CO2) emissions associated with conventional coal-to-aromatics (CTA) processes. This study conducted a detailed process simulation and optimization of key parameters to determine the aromatic production route with the lowest carbon emission. A comprehensive technical and economic analysis, along with an environmental assessment, was carried out to compare the proposed processes with existing ones. The results indicate that the NG-CTA-DS process has demonstrated superior techno-economic performance and environmental evaluation. It achieved an elemental carbon utilization of 85.95 %, an energy efficiency of 78.80 %, a reduced CO2 emission of 3.65 kg/kg-aromatics, and a production cost of only 1018.87 M$. Therefore, it is evident that the proposed NGCTA-DS process holds significant potential to enhance the technical, economic, and environmental performance compared to the conventional process, making it a promising candidate for industrialization.
引用
收藏
页数:13
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