Flower-like WO3 Nanorod Structures Modified with MoS2 Quantum Dots for Low-Temperature Acetone Detection

被引:1
作者
Shang, Jichao [1 ,2 ,3 ]
Zhou, Mingyue [1 ,2 ]
Xie, Fuwei [3 ]
Li, Shuqi [3 ]
Tu, Shiyu [3 ]
Liu, Xiangrui [3 ]
Zhang, Lu [1 ,2 ]
机构
[1] Xinjiang Univ, Sch Pharmaceut Sci, Urumqi 830017, Peoples R China
[2] Xinjiang Univ, Inst Mat Med, Urumqi 830017, Peoples R China
[3] Xinjiang Univ, Coll Life Sci & Technol, Xinjiang Key Lab Biol Resources & Genet Engn, Urumqi 830046, Peoples R China
关键词
acetone; WO3; MoS2; gas sensors; quantum dots; n-n junction; SENSOR; SENSITIVITY; NANOSHEETS; ETHANOL; BREATH;
D O I
10.1021/acsanm.4c06344
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
As a prevalent volatile organic compound (VOC), acetone plays a significant role in diverse domains, such as environmental protection, industrial production, and medical diagnosis. However, if acetone is not adequately monitored and disposed of, it can result in immeasurable adverse effects on human health and the natural environment. Therefore, it is essential to realize the highly sensitive, convenient, and efficient real-time detection of acetone. In this study, MoS2 quantum dots (QDs) were modified on flower-like WO3 nanorod structure through the hydrothermal approach to fabricate a WO3/MoS2 sensor. The sensing performance of the sensor for acetone was investigated. The results showed that the sensor had a response value of 14.96 for 30 ppm of acetone gas at optimum operating temperature (132 degrees C), which was 3.2 times the performance of a pure WO3 gas sensor. The response of the WO3/MoS2 sensor was reduced by only 20% under a relative humidity of 85%. Besides, the sensor still maintained a high response (11.25 for 30 ppm) under high curvature conditions (120 degrees). Finally, the sensitization effects of MoS2 QDs, including the formation of n-n heterojunction with WO3 and the catalytic overflow of oxygen species, were discussed in detail. This study provides a valuable reference for the construction of low-temperature and high-performance gas sensors based on QD-sensitized metal oxide nanomaterials.
引用
收藏
页码:28818 / 28828
页数:11
相关论文
共 56 条
  • [41] Synthesis and excellent acetone sensing properties of porous WO3 nanofibers
    Wei, Shaohong
    Zhao, Guoyan
    Du, Weimin
    Tian, Qingqing
    [J]. VACUUM, 2016, 124 : 32 - 39
  • [42] Interfacial Charge Transfer in MoS2/TiO2 Heterostructured Photocatalysts: The Impact of Crystal Facets and Defects
    Wei, Tingcha
    Lau, Woon Ming
    An, Xiaoqiang
    Yu, Xuelian
    [J]. MOLECULES, 2019, 24 (09):
  • [43] Visual chemiresistive dual-mode sensing platform based on SnS2/Ti3C2 MXene Schottky junction for acetone detection at room temperature
    Wu, Qingjin
    Feng, Zeguo
    Wang, Ziheng
    Peng, Zhengchun
    Zhang, Lu
    Li, Yingchun
    [J]. TALANTA, 2023, 253
  • [44] MoS2 quantum dots interspersed WO3 nanoplatelet arrays with enhanced photoelectrochemical activity
    Xiao, Yong-Hao
    Zhang, Wei-De
    [J]. ELECTROCHIMICA ACTA, 2017, 252 : 416 - 423
  • [45] Triethylamine Gas Sensors Based on BiOBr Microflowers Decorated with ZnO
    Xu, Xiaoli
    Wang, Xiaoping
    Liu, Wangwang
    Wang, Shengyi
    Jiang, Hongtao
    Ma, Shuyi
    Yuan, Fangqiang
    Ma, Nina
    [J]. ACS APPLIED NANO MATERIALS, 2022, 5 (10) : 15837 - 15846
  • [46] Platinum single atoms on tin oxide ultrathin films for extremely sensitive gas detection
    Xu, Yongshan
    Zheng, Wei
    Liu, Xianghong
    Zhang, Liqiang
    Zheng, Lingli
    Yang, Chen
    Pinna, Nicola
    Zhang, Jun
    [J]. MATERIALS HORIZONS, 2020, 7 (06) : 1519 - 1527
  • [47] Three-Dimensional MoS2/Reduced Graphene Oxide Nanosheets/Graphene Quantum Dots Hybrids for High-Performance Room-Temperature NO2 Gas Sensors
    Yang, Cheng
    Wang, Yanyan
    Wu, Zhekun
    Zhang, Zhanbo
    Hu, Nantao
    Peng, Changsi
    [J]. NANOMATERIALS, 2022, 12 (06)
  • [48] Characteristics of binary WO3@CuO and ternary WO3@PDA@CuO based on impressive sensing acetone odor
    Yang, Fuchao
    Wang, Fengyi
    Guo, Zhiguang
    [J]. JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2018, 524 : 32 - 41
  • [49] Metal Oxide Based Heterojunctions for Gas Sensors: A Review
    Yang, Shulin
    Lei, Gui
    Xu, Huoxi
    Lan, Zhigao
    Wang, Zhao
    Gu, Haoshuang
    [J]. NANOMATERIALS, 2021, 11 (04)
  • [50] Synthesis of Ag quantum dots sensitized WO3 nanosheets and their enhanced acetone sensing properties
    Yin, Mingli
    Yu, Lingmin
    Liu, Shengzhong
    [J]. MATERIALS LETTERS, 2017, 186 : 66 - 69