Reentrant multiple-<bold>q</bold> magnetic order and a "spin meta-cholesteric" phase in Sr3Fe2O7

被引:1
作者
Andriushin, N. D. [1 ]
Muller, J. [2 ]
Pavlovskii, N. S. [1 ]
Grumbach, J. [1 ]
Granovsky, S. [1 ]
Tymoshenko, Y. V. [1 ]
Zaharko, O. [3 ]
Ivanov, A. [4 ]
Ollivier, J. [4 ]
Doerr, M. [1 ]
Keimer, B. [5 ]
Mostovoy, M. [2 ]
Inosov, D. S. [1 ,6 ]
Peets, D. C. [1 ,5 ]
机构
[1] Tech Univ Dresden, Inst Festkorper & Materialphys, Dresden, Germany
[2] Univ Groningen, Zernike Inst Adv Mat, Groningen, Netherlands
[3] Paul Scherrer Inst, Lab Neutron Scattering & Imaging, Villigen, Switzerland
[4] Inst Laue Langevin, Grenoble, France
[5] Max Planck Inst Festkorperforsch, Stuttgart, Germany
[6] Tech Univ Dresden, Wurzburg Dresden Cluster Excellence Complex & Topo, Dresden, Germany
关键词
CRYSTALS; STATE;
D O I
10.1038/s41535-024-00698-4
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Topologically nontrivial magnetic structures such as skyrmion lattices are well known in materials lacking lattice inversion symmetry, where antisymmetric exchange interactions are allowed. Only recently, topological multi-q magnetic textures that spontaneously break the chiral symmetry, for example, three-dimensional hedgehog lattices, were discovered in centrosymmetric compounds, where they are instead driven by frustrated interactions. Here we show that the bilayer perovskite Sr3Fe2O7, previously believed to adopt a simple single-q spin-helical order, hosts two distinct types of multi-q spin textures. Its ground state represents a novel multi-q spin texture with unequally intense spin modulations at the two ordering vectors. This is followed in temperature by a new "spin meta-cholesteric" phase, in which the chiral symmetry is spontaneously broken along one of the crystal directions, but the weaker orthogonal modulation melts, giving rise to intense short-range dynamical fluctuations. Shortly before the transition to the paramagnetic state, vortex-crystal order spanned by two equivalent q vectors emerges. This renders Sr3Fe2O7 an ideal material to study transitions among multiple-q spin textures in a centrosymmetric host.
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页数:6
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