A single nanophotonic platform for producing circularly polarized white light from non-chiral emitters

被引:5
作者
Mendoza-Carreno, Jose [1 ]
Bertucci, Simone [2 ,3 ]
Garbarino, Mauro [2 ,3 ]
Cirignano, Matilde [2 ]
Fiorito, Sergio [2 ]
Lova, Paola [3 ]
Garriga, Miquel [1 ]
Alonso, Maria Isabel [1 ]
Di Stasio, Francesco [2 ]
Mihi, Agustin [1 ]
机构
[1] Inst Mat Sci Barcelona ICMAB CSIC, Campus UAB, Bellaterra, Spain
[2] Ist Italiano Tecnol, Photon Nanomat, Genoa, Italy
[3] Univ Genoa, Dipartimento Chim & Chim Industriale, Genoa, Italy
基金
欧洲研究理事会;
关键词
CORE-SHELL NANOCRYSTALS; EMISSION;
D O I
10.1038/s41467-024-54792-z
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Direct manipulation of light spin-angular momentum is desired in optoelectronic applications such as, displays, telecommunications, or imaging. Generating polarized light from luminophores avoids using optical components that cause brightness losses and hamper on-chip integration of light sources. Endowing chirality to achiral emitters for direct generation of polarized light benefits from existing materials and can be achieved by chiral nanophotonics. However, most chiral nanostructures operate in narrow wavelength ranges and involve nanofabrication processes incompatible with high-throughput production. Here, a single nanophotonic architecture is designed to sustain chiroptical resonances along the visible spectrum. This platform, fabricated with scalable soft-nanoimprint lithography transfers its chirality to conventional emitters (CdSe/CdS nanoplatelets, CdSe/CdS quantum dots, CsPbBr3, CsPbI3 perovskite nanocrystals and F8BT) placed atop, achieving a high dissymmetry emission factor (g(lum) > 1). The dynamics study suggests enhanced out-coupling efficiency for one helicity by the photonic structure. Finally, a white light-emitting blend containing different emitters shows simultaneous dissymmetric emission values along the visible spectrum with this chiral nanophotonic platform.
引用
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页数:11
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