Discovery of superconductivity and electron-phonon drag in the non-centrosymmetric Weyl semimetal LaRhGe3

被引:1
作者
Oudah, Mohamed [1 ]
Kung, Hsiang-Hsi [1 ]
Sahu, Samikshya [1 ,2 ]
Heinsdorf, Niclas [1 ,2 ,3 ]
Schulz, Armin [3 ]
Philippi, Kai [3 ]
Sanchez, Marta-Villa De Toro [4 ]
Cai, Yipeng [4 ]
Kojima, Kenji [1 ,4 ]
Schnyder, Andreas P. [3 ]
Takagi, Hidenori [3 ]
Keimer, Bernhard [3 ]
Bonn, Doug A. [1 ,2 ]
Hallas, Alannah M. [1 ,2 ,5 ]
机构
[1] Univ British Columbia, Stewart Blusson Quantum Matter Inst, Vancouver, BC, Canada
[2] Univ British Columbia, Dept Phys & Astron, Vancouver, BC, Canada
[3] Max Planck Inst Solid State Res, Stuttgart, Germany
[4] TRIUMF, Vancouver, BC, Canada
[5] Canadian Inst Adv Res, Toronto, ON, Canada
基金
加拿大自然科学与工程研究理事会;
关键词
GENERALIZED GRADIENT APPROXIMATION; TOTAL-ENERGY CALCULATIONS; MAGNETORESISTANCE; DYNAMICS; GE;
D O I
10.1038/s41535-024-00686-8
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We present an exploration of the effect of electron-phonon coupling and broken inversion symmetry on the electronic and thermal properties of the semimetal LaRhGe3. Our transport measurements reveal evidence for electron-hole compensation at low temperatures, resulting in a large magnetoresistance of 3000% at 1.8 K and 14 T. The carrier concentration is on the order of 10(21)/cm(3) with high carrier mobilities of 2000 cm(2)/Vs. When coupled to our theoretical demonstration of symmetry-protected almost movable Weyl nodal lines, we conclude that LaRhGe3 supports a Weyl semimetallic state. We discover superconductivity in this compound with a T-c of 0.39(1) K and B-c(0) of 2.2(1) mT, with evidence from specific heat and transverse-field muon spin relaxation. We find an exponential dependence in the normal state electrical resistivity below similar to 50 K, while Seebeck coefficient and thermal conductivity measurements each reveal a prominent peak at low temperatures, indicative of strong electron-phonon interactions. To this end, we examine the temperature-dependent Raman spectra of LaRhGe3 and find that the lifetime of the lowest energy A(1) phonon is dominated by phonon-electron scattering instead of anharmonic decay. We conclude that LaRhGe3 has strong electron-phonon coupling in the normal state, while the superconductivity emerges from weak electron-phonon coupling. These results open up the investigation of electron-phonon interactions in the normal state of superconducting non-centrosymmetric Weyl semimetals.
引用
收藏
页数:11
相关论文
共 80 条
  • [1] Large, non-saturating magnetoresistance in WTe2
    Ali, Mazhar N.
    Xiong, Jun
    Flynn, Steven
    Tao, Jing
    Gibson, Quinn D.
    Schoop, Leslie M.
    Liang, Tian
    Haldolaarachchige, Neel
    Hirschberger, Max
    Ong, N. P.
    Cava, R. J.
    [J]. NATURE, 2014, 514 (7521) : 205 - +
  • [2] SOME EFFECTS OF PHONON DYNAMICS ON ELECTRON LIFETIME, MASS RENORMALIZATION, AND SUPERCONDUCTING TRANSITION-TEMPERATURE
    ALLEN, PB
    SILBERGLITT, R
    [J]. PHYSICAL REVIEW B, 1974, 9 (11) : 4733 - 4741
  • [3] Specific heat and μSR study on the noncentrosymmetric superconductor LaRhSi3
    Anand, V. K.
    Hillier, A. D.
    Adroja, D. T.
    Strydom, A. M.
    Michor, H.
    McEwen, K. A.
    Rainford, B. D.
    [J]. PHYSICAL REVIEW B, 2011, 83 (06)
  • [4] Weyl and Dirac semimetals in three-dimensional solids
    Armitage, N. P.
    Mele, E. J.
    Vishwanath, Ashvin
    [J]. REVIEWS OF MODERN PHYSICS, 2018, 90 (01)
  • [5] Extremely large magnetoresistance from electron-hole compensation in the nodal-loop semimetal ZrP2
    Bannies, J.
    Razzoli, E.
    Michiardi, M.
    Kung, H-H
    Elfimov, I. S.
    Yao, M.
    Fedorov, A.
    Fink, J.
    Jozwiak, C.
    Bostwick, A.
    Rotenberg, E.
    Damascelli, A.
    Felser, C.
    [J]. PHYSICAL REVIEW B, 2021, 103 (15)
  • [6] Heavy fermion superconductivity and magnetic order in noncentrosymmetric CePt3Si -: art. no. 027003
    Bauer, E
    Hilscher, G
    Michor, H
    Paul, C
    Scheidt, EW
    Gribanov, A
    Seropegin, Y
    Noël, H
    Sigrist, M
    Rogl, P
    [J]. PHYSICAL REVIEW LETTERS, 2004, 92 (02) : 4
  • [7] Bauer E, 2012, LECT NOTES PHYS, V847, P1, DOI 10.1007/978-3-642-24624-1
  • [8] Experimental study of transport properties of Weyl semimetal LaAlGe thin films grown by molecular beam epitaxy
    Bhattarai, Niraj
    Forbes, Andrew W.
    Gassen, Christopher
    Saqat, Raghad S. H.
    Pegg, Ian L.
    Philip, John
    [J]. JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A, 2021, 39 (06):
  • [9] Phonon anharmonicities in graphite and graphene
    Bonini, Nicola
    Lazzeri, Michele
    Marzari, Nicola
    Mauri, Francesco
    [J]. PHYSICAL REVIEW LETTERS, 2007, 99 (17)
  • [10] Topological semimetals
    Burkov, A. A.
    [J]. NATURE MATERIALS, 2016, 15 (11) : 1145 - 1148