CuS-NiTe2 embedded phosphorus-doped graphene oxide catalyst for evaluating hydrogen evolution reaction

被引:1
|
作者
Parvaz, Sedigheh [1 ]
Vandishi, Zahra Talebi [1 ]
Ensafi, Ali A. [1 ,2 ]
Mousaabadi, Kimia Zarean [1 ]
机构
[1] Isfahan Univ Technol, Dept Chem, Esfahan 8415683111, Iran
[2] Univ Arkansas, Dept Chem & Biochem, Fayetteville, AR 72701 USA
来源
SCIENTIFIC REPORTS | 2024年 / 14卷 / 01期
关键词
Hydrogen evolution reaction; Bimetallic; Telluro-sulfide; Graphene oxide; Electrocatalyst; EFFICIENT; ELECTROCATALYST; NANOSHEETS; OXIDATION; FRAMEWORK; ALLOY;
D O I
10.1038/s41598-024-78870-w
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
The hydrogen evolution reaction (HER), a crucial half-reaction in the water-splitting process, is hindered by slow kinetics, necessitating efficient electrocatalysts to lower overpotential and enhance energy conversion efficiency. Transition-metal electrode materials, renowned for their robustness and effectiveness, have risen to prominence as primary contenders in the field of energy conversion and storage research. In this investigation, we delve into the capabilities of transition metals when employed as catalysts for the HER. Furthermore, we turn our attention to carbon nanomaterials like graphene, which have exhibited tremendous potential as top-performing electrocatalysts. Nevertheless, advancements are indispensable to expand their utility and versatility. One such enhancement involves the integration of phosphorus-doped graphene. Our research focuses on the synthesis of CuS-NiTe2/PrGO, a nanocomposite with a crystalline structure, through a straightforward method. This nanocomposite exhibits enhanced catalytic activity for the HER, boasting a Tafel slope of 57 mV dec-1 in an acidic environment. Consequently, our findings present a straightforward and efficient approach to developing high-performance electrocatalysts for HER.
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页数:12
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