High-Performance Red Transparent Quantum Dot Light-Emitting Diodes via Fully Solution-Processed MXene/Ag NWs Top Electrode

被引:3
作者
Su, Daojian [1 ,2 ]
Ding, Ting [2 ]
Gao, Peili [2 ]
Liu, Hang [2 ]
Song, Yinman [2 ]
Yuan, Guoqiang [1 ,3 ]
He, Xin [1 ,3 ]
Meng, Fanyuan [1 ,3 ]
Wang, Shuangpeng [2 ]
机构
[1] Wuyi Univ, Sch Appl Phys & Mat, Jiangmen 529020, Peoples R China
[2] Univ Macau, Inst Appl Phys & Mat Engn, Joint Key Lab, Minist Educ, Ave Univ, Taipa 999078, Macau, Peoples R China
[3] Jiangmen Key Lab Micronano Funct Mat & Devices, Jiangmen 529020, Peoples R China
关键词
transparent electrodes; MXene; silver nanowires; interface engineering; organic light-emitting diodes; EMISSION;
D O I
10.1021/acsami.4c11431
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
The integration of high-performance transparent top electrodes with the functional layers of transparent quantum dot light-emitting diodes (T-QLEDs) poses a notable challenge. This study presents a composite transparent top electrode composed of MXene and Ag NWs. The composite electrode demonstrates exceptional transparency (84.6% at 620 nm) and low sheet resistance (16.07 Omega sq(-1)), rendering it suitable for integration into T-QLEDs. The inclusion of MXene nanosheets in the composite electrode serves a dual role: adjusting the work function to enhance electron injection efficiency and enhancing the interface between Ag NWs and the emissive layer, thereby mitigating the common issue of interfacial resistance in conventional transparent electrodes. This strategic amalgamation results in notable improvements in device performance, yielding a maximum current efficiency of 23.12 cd A(-1), an external quantum efficiency of 13.98%, and a brightness of 21,015 cd m(-2). These performance metrics surpass those achieved by T-LEDs employing pristine Ag NW electrodes. This study offers valuable insights into T-QLED device advancement and provides a promising approach for transparent electrode fabrication in optoelectronic applications.
引用
收藏
页码:54189 / 54198
页数:10
相关论文
共 51 条
[1]   High efficiency quantum dot light emitting diodes from positive aging [J].
Acharya, Krishna P. ;
Titov, Alexandre ;
Hyvonen, Jake ;
Wang, Chenggong ;
Tokarz, Jean ;
Holloway, Paul H. .
NANOSCALE, 2017, 9 (38) :14451-14457
[2]   Shelf-Stable Quantum-Dot Light-Emitting Diodes with High Operational Performance [J].
Chen, Desui ;
Chen, Dong ;
Dai, Xingliang ;
Zhang, Zhenxing ;
Lin, Jian ;
Deng, Yunzhou ;
Hao, Yanlei ;
Zhang, Ci ;
Zhu, Haiming ;
Gao, Feng ;
Jin, Yizheng .
ADVANCED MATERIALS, 2020, 32 (52)
[3]   On the degradation mechanisms of quantum-dot light-emitting diodes [J].
Chen, Song ;
Cao, Weiran ;
Liu, Taili ;
Tsang, Sai-Wing ;
Yang, Yixing ;
Yan, Xiaolin ;
Qian, Lei .
NATURE COMMUNICATIONS, 2019, 10 (1)
[4]   Efficient and Stable Quantum-Dot Light-Emitting Diodes Enabled by Tin Oxide Multifunctional Electron Transport Layer [J].
Chen, Zinan ;
Chen, Shuming .
ADVANCED OPTICAL MATERIALS, 2022, 10 (05)
[5]   Extremely Vivid, Highly Transparent, and Ultrathin Quantum Dot Light-Emitting Diodes [J].
Choi, Moon Kee ;
Yang, Jiwoong ;
Kim, Dong Chan ;
Dai, Zhaohe ;
Kim, Junhee ;
Seung, Hyojin ;
Kale, Vinayak S. ;
Sung, Sae Jin ;
Park, Chong Rae ;
Lu, Nanshu ;
Hyeon, Taeghwan ;
Kim, Dae-Hyeong .
ADVANCED MATERIALS, 2018, 30 (01)
[6]   Observation and Suppression of Stacking Interface States in Sandwich-Structured Quantum Dot Light-Emitting Diodes [J].
Dong, Jia-Yi ;
Ng, Kar Wei ;
Song, Yin-Man ;
Li, Jie-Lei ;
Kong, You-Chao ;
Wang, Meng-Wei ;
Xu, Jin-Cheng ;
Li, Lin ;
Chen, Shi ;
Tang, Zi-Kang ;
Wang, Shuang-Peng .
ACS APPLIED MATERIALS & INTERFACES, 2021, 13 (47) :56630-56637
[7]   Highly Efficient Red Quantum Dot Light-Emitting Diodes by Balancing Charge Injection and Transport [J].
Fang, Yunfeng ;
Bai, Penglong ;
Li, Jiayi ;
Xiao, Binbin ;
Wang, Yiqing ;
Wang, Yanping .
ACS APPLIED MATERIALS & INTERFACES, 2022, 14 (18) :21263-21269
[8]   Architectural Engineering of Nanowire Network Fine Pattern for 30 μm Wide Flexible Quantum Dot Light-Emitting Diode Application [J].
Fang, Yunsheng ;
Ding, Ke ;
Wu, Zhicong ;
Chen, Hongting ;
Li, Wenbo ;
Zhao, Sheng ;
Zhang, Yanli ;
Wang, Lei ;
Zhou, Jun ;
Hu, Bin .
ACS NANO, 2016, 10 (11) :10023-10030
[9]   Highly Sensitive Pseudocapacitive Iontronic Pressure Sensor with Broad Sensing Range [J].
Gao, Libo ;
Wang, Meng ;
Wang, Weidong ;
Xu, Hongcheng ;
Wang, Yuejiao ;
Zhao, Haitao ;
Cao, Ke ;
Xu, Dandan ;
Li, Lei .
NANO-MICRO LETTERS, 2021, 13 (01)
[10]   Changes in Hole and Electron Injection under Electrical Stress and the Rapid Electroluminescence Loss in Blue Quantum-Dot Light-Emitting Devices [J].
Ghorbani, Atefeh ;
Chen, Junfei ;
Chun, Peter ;
Lyu, Quan ;
Cotella, Giovanni ;
Aziz, Hany .
SMALL, 2024, 20 (01)