High-Performance Red Transparent Quantum Dot Light-Emitting Diodes via Fully Solution-Processed MXene/Ag NWs Top Electrode

被引:0
|
作者
Su, Daojian [1 ,2 ]
Ding, Ting [2 ]
Gao, Peili [2 ]
Liu, Hang [2 ]
Song, Yinman [2 ]
Yuan, Guoqiang [1 ,3 ]
He, Xin [1 ,3 ]
Meng, Fanyuan [1 ,3 ]
Wang, Shuangpeng [2 ]
机构
[1] Wuyi Univ, Sch Appl Phys & Mat, Jiangmen 529020, Peoples R China
[2] Univ Macau, Inst Appl Phys & Mat Engn, Joint Key Lab, Minist Educ, Ave Univ, Taipa 999078, Macau, Peoples R China
[3] Jiangmen Key Lab Micronano Funct Mat & Devices, Jiangmen 529020, Peoples R China
关键词
transparent electrodes; MXene; silver nanowires; interface engineering; organic light-emitting diodes; EMISSION;
D O I
10.1021/acsami.4c11431
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
The integration of high-performance transparent top electrodes with the functional layers of transparent quantum dot light-emitting diodes (T-QLEDs) poses a notable challenge. This study presents a composite transparent top electrode composed of MXene and Ag NWs. The composite electrode demonstrates exceptional transparency (84.6% at 620 nm) and low sheet resistance (16.07 Omega sq(-1)), rendering it suitable for integration into T-QLEDs. The inclusion of MXene nanosheets in the composite electrode serves a dual role: adjusting the work function to enhance electron injection efficiency and enhancing the interface between Ag NWs and the emissive layer, thereby mitigating the common issue of interfacial resistance in conventional transparent electrodes. This strategic amalgamation results in notable improvements in device performance, yielding a maximum current efficiency of 23.12 cd A(-1), an external quantum efficiency of 13.98%, and a brightness of 21,015 cd m(-2). These performance metrics surpass those achieved by T-LEDs employing pristine Ag NW electrodes. This study offers valuable insights into T-QLED device advancement and provides a promising approach for transparent electrode fabrication in optoelectronic applications.
引用
收藏
页码:54189 / 54198
页数:10
相关论文
共 50 条
  • [1] High performance, top-emitting, quantum dot light-emitting diodes with all solution-processed functional layers
    Tang, Zhaobing
    Lin, Jie
    Wang, Lishuang
    Lv, Ying
    Hu, Yongsheng
    Fan, Yi
    Guo, Xiaoyang
    Zhao, Jialong
    Wang, Yunjun
    Liu, Xingyuan
    JOURNAL OF MATERIALS CHEMISTRY C, 2017, 5 (35) : 9138 - 9145
  • [2] Fully solution-processed red tandem quantum dot light-emitting diodes with an EQE exceeding 35%
    Sun, Yuhan
    Han, Changfeng
    Li, Ruifeng
    Xiang, Chaoyu
    Zhang, Ting
    Qian, Lei
    JOURNAL OF MATERIALS CHEMISTRY C, 2024, 12 (27) : 10053 - 10060
  • [3] Solution-processed, high-performance light-emitting diodes based on quantum dots
    Xingliang Dai
    Zhenxing Zhang
    Yizheng Jin
    Yuan Niu
    Hujia Cao
    Xiaoyong Liang
    Liwei Chen
    Jianpu Wang
    Xiaogang Peng
    Nature, 2014, 515 : 96 - 99
  • [4] Solution-processed, high-performance light-emitting diodes based on quantum dots
    Dai, Xingliang
    Zhang, Zhenxing
    Jin, Yizheng
    Niu, Yuan
    Cao, Hujia
    Liang, Xiaoyong
    Chen, Liwei
    Wang, Jianpu
    Peng, Xiaogang
    NATURE, 2014, 515 (7525) : 96 - 99
  • [5] Advances in Solution-Processed Blue Quantum Dot Light-Emitting Diodes
    Li, Sheng-Nan
    Pan, Jia-Lin
    Yu, Yan-Jun
    Zhao, Feng
    Wang, Ya-Kun
    Liao, Liang-Sheng
    NANOMATERIALS, 2023, 13 (10)
  • [6] Improving the Performance of Solution-Processed Quantum Dot Light-Emitting Diodes via a HfOx Interfacial Layer
    Jeong, Jun Hyung
    Kim, Min Gye
    Ma, Jin Hyun
    Park, Min Ho
    Ha, Hyoun Ji
    Kang, Seong Jae
    Maeng, Min-Jae
    Kim, Young Duck
    Park, Yongsup
    Kang, Seong Jun
    MATERIALS, 2022, 15 (24)
  • [7] Solution-processed PEDOT:PSS:GO/Ag NWs composite electrode for flexible organic light-emitting diodes
    Du, Hui
    Guo, Yangyang
    Cui, Dongyue
    Li, Shuhong
    Wang, Wenjun
    Liu, Yunlong
    Yao, Yicun
    Zhao, Ling
    Dong, Xiaochen
    SPECTROCHIMICA ACTA PART A-MOLECULAR AND BIOMOLECULAR SPECTROSCOPY, 2021, 248 (248)
  • [8] Solution-processed transparent blue organic light-emitting diodes with graphene as the top cathode
    Chang, Jung-Hung
    Lin, Wei-Hsiang
    Wang, Po-Chuan
    Taur, Jieh-I
    Ku, Ting-An
    Chen, Wei-Ting
    Yan, Shiang-Jiuan
    Wu, Chih-I
    SCIENTIFIC REPORTS, 2015, 5
  • [9] Multifunctional Dendrimer Ligands for High Efficiency, Solution-Processed Quantum Dot Light-Emitting Diodes
    Cho, Ikjun
    Jung, Heeyoung
    Jeong, Byeong Guk
    Chang, Jun Hyuk
    Kim, Younghoon
    Char, Kookheon
    Lee, Doh C.
    Lee, Changhee
    Cho, Jinhan
    Bae, Wan Ki
    ACS NANO, 2017, 11 (01) : 684 - 692
  • [10] Solution-processed transparent blue organic light-emitting diodes with graphene as the top cathode
    Jung-Hung Chang
    Wei-Hsiang Lin
    Po-Chuan Wang
    Jieh-I Taur
    Ting-An Ku
    Wei-Ting Chen
    Shiang-Jiuan Yan
    Chih-I Wu
    Scientific Reports, 5