Current status and research progress of recovery and recycling of electrolyte and anode materials of spent lithium-ion batteries

被引:0
作者
Yang, Yakai [1 ]
Zhang, Hao [1 ]
Song, Dongqi [1 ]
Wan, Hao [2 ]
Guo, Hui [1 ]
Cao, Yijun [1 ,2 ]
机构
[1] School of Chemical Engineering, Zhengzhou University, Zhengzhou
[2] Zhongyuan Critical Metals Laboratory, Zhengzhou University, Zhengzhou
来源
Zhongnan Daxue Xuebao (Ziran Kexue Ban)/Journal of Central South University (Science and Technology) | 2024年 / 55卷 / 11期
基金
中国国家自然科学基金;
关键词
anode; electrolyte; graphite; recovery; regeneration; spent lithium-ion battery;
D O I
10.11817/j.issn.1672-7207.2024.11.027
中图分类号
学科分类号
摘要
The research on the recovery of cathode materials from spent lithium-ion batteries was extensively studied. The current status of electrolyte and anode material recovery and utilization were reviewed. The pretreatment of spent LIBs was firstly reviewed. Then, the collection of electrolyte and the conversion and recovery method of lithium salt were discussede. Moreover, the research status of regenerated graphite by hydrometallurgy, pyrometallurgy and the combined process was summarized. Besides, research on the regeneration of anode materials into other functional materials such as graphene, adsorbents and catalysts was also reviewed. Finally, the challenges and opportunities for the recycling of anode materials were summarized, aiming to provide guidance for the recycling of electrolyte and anode materials of spent LIBs. © 2024 Central South University. All rights reserved.
引用
收藏
页码:4318 / 4331
页数:13
相关论文
共 75 条
[1]  
FAN Xinming, HU Guorong, ZHANG Bao, Et al., Crack-free single-crystalline Ni-rich layered NCM cathode enable superior cycling performance of lithium-ion batteries, Nano Energy, 70, (2020)
[2]  
HARPER G, SOMMERVILLE R, KENDRICK E, Et al., Recycling lithium-ion batteries from electric vehicles[J], Nature, 575, 7781, (2019)
[3]  
ZHANG Duchao, LI Tingying, WANG Hao, Et al., Removal of impurity elements from waste lithium-ion batteries powder by oxidation roasting, cyclic leaching, and precipitation method[J], Journal of Central South University, 30, 7, (2023)
[4]  
YU Jiadong, HE Yaqun, GE Zhenzhou, Et al., A promising physical method for recovery of LiCoO<sub>2</sub> and graphite from spent lithium-ion batteries: grinding flotation[J], Separation and Purification Technology, 190, (2018)
[5]  
HU Huakun, XUE Wendong, JIANG Peng, Et al., Research progress of safety additives for lithium ion batteries, Chemical Industry and Engineering Progress, 41, 10, pp. 5441-5455, (2022)
[6]  
GUO Yang, LI Feng, ZHU Haochen, Et al., Leaching lithium from the anode electrode materials of spent lithium-ion batteries by hydrochloric acid (HCl)[J], Waste Management, 51, (2016)
[7]  
CHENG Qian, MARCHETTI B, CHEN Xuanyi, Et al., Separation, purification, regeneration and utilization of graphite recovered from spent lithium-ion batteries: a review, Journal of Environmental Chemical Engineering, 10, 2, (2022)
[8]  
ZHANG Guangwen, HE Yaqun, FENG Yi, Et al., Pyrolysis-ultrasonic-assisted flotation technology for recovering graphite and LiCoO<sub>2</sub> from spent lithium-ion batteries, ACS Sustainable Chemistry & Engineering, 6, 8, pp. 10896-10904, (2018)
[9]  
ROY J J, RAROTRA S, KRIKSTOLAITYTE V, Et al., Green recycling methods to treat lithium-ion batteries E-waste: a circular approach to sustainability, Advanced Materials, 34, 25, (2022)
[10]  
GOLMOHAMMADZADEH R, FARAJI F, JONG B, Et al., Current challenges and future opportunities toward recycling of spent lithium-ion batteries, Renewable and Sustainable Energy Reviews, 159, (2022)