Reactive spark plasma sintering and luminescence properties of Gd2O2S:Tb nanocrystalline phosphor

被引:0
作者
Shichalin, O. O. [1 ,2 ]
Shi, Yun [3 ,4 ]
Vornovskikh, A. A. [1 ]
Kornakova, Z. E. [1 ,2 ]
Amosov, A. V. [5 ]
Belov, A. A. [1 ]
Seroshtan, A. I. [1 ,2 ]
Ivanov, N. P. [1 ]
Marmaza, P. A. [1 ,2 ]
Buravlev, I. Yu [1 ]
Starev, D. S. [1 ,6 ]
Kosyanov, D. Yu [1 ,5 ]
Papynov, E. K. [1 ]
机构
[1] Far Eastern Fed Univ, 10 Ajax Bay, Russky Isl, Vladivostok 690922, Russia
[2] Sakhalin State Univ, 33 Kommunistichesky Ave, Yuzhno Sakhalinsk 693000, Russia
[3] Chinese Acad Sci, Shanghai Inst Ceram, 585 He shuo Rd, Shanghai 201899, Peoples R China
[4] Univ Chinese Acad Sci, Ctr Mat Sci & Optoelect Engn, Beijing 100049, Peoples R China
[5] RAS, Inst Automat & Control Proc FEB, 5 Radio St, Vladivostok 690041, Russia
[6] Shenzhen MSU BIT Univ, Dept Engn, Int Univ Pk Rd,Dayun New Town, Shenzhen 51817, Guangdong, Peoples R China
基金
俄罗斯科学基金会;
关键词
Reactive synthesis; Spark plasma sintering (SPS); Nanocrystalline phosphors; SCINTILLATION PROPERTIES; SOLVOTHERMAL SYNTHESIS; OPTICAL-PROPERTIES; LN(2)O(2)S LN; SPS; EMISSION; TB; GD; LA; TEMPERATURE;
D O I
10.1016/j.optmat.2024.116312
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Gd2O2S:Tb is promising for energy-efficient lighting and display applications. This work explores the use of reactive spark plasma sintering (SPS) to synthesis Gd2O2S:Tb nanocrystalline phosphor. It allows to significantly simplify the technological process in comparison with traditional multi-stage liquid-phase synthesis. As-sintered Gd2O2S:Tb demonstrated average crystallite size of 26 nm and secondary particle size of 26 mu m. Bright green emission occurs at 545 nm under UV excitation of 245 nm. Average fluorescence lifetime was 0.656 ms. Further consolidation of the Gd2O2S:Tb prepared via reactive SPS can also be expected to yield highly dense ceramics. The innovative reactive synthesis strategies provide valuable insights into the design and development of highperformance luminescent ceramics.
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页数:8
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