Advanced X-ray spectroscopies: Unveiling chemical reaction mechanism in photo/electrocatalytic water splitting

被引：0

作者：

Shen, Lifu ^{[1
]}

Yu, Pengfei ^{[2
]}

Meng, Jianwei ^{[2
]}

Liu, Xiaosong ^{[3
]}

Weng, Tsu-Chien ^{[1
,2
]}

机构：

[1] ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 200100, Peoples R China

[2] ShanghaiTech Univ, Ctr Transformat Sci, Shanghai 200100, Peoples R China

[3] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Anhui, Peoples R China

来源：

MATERIALS TODAY CHEMISTRY | 2024年 / 42卷

基金：

中国国家自然科学基金;

关键词：

X-ray spectroscopy; In-situ / operando measurement; Spectroscopic imaging; Photo/electrocatalysis; Water splitting; HYDROGEN-EVOLUTION REACTION; PHOTOELECTRON-SPECTROSCOPY; ELECTRONIC-STRUCTURE; OXYGEN REDUCTION; WORKING CATALYST; TRANSITION-METAL; TOOL; ELECTROCHEMISTRY; SPECTRA; SURFACE;

D O I：

10.1016/j.mtchem.2024.102397

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The challenge of detecting intermediates in photo/electrocatalytic water splitting hinges critically on a profound understanding of processes across multiple spatial and temporal scales, encompassing electron excitation, electron transfer, interfacial reaction kinetics and so on. Advanced X-ray spectroscopies are powerful tools for analyzing complex processes at various scales. They offer non-destructive insights into electron dynamics, local structures, crystal lattices, and material distributions through absorption and imaging. This article provides an overview of the diverse applications of X-ray spectroscopies in the study of photo/electrocatalytic water splitting. It begins by introducing the fundamental principles of photo/electrocatalytic reactions for water splitting. Subsequently, it discusses the successful application of X-ray spectroscopic tools on the scales of energy resolution, temporal resolution, and spatial resolution in elucidating the mechanisms of chemical reactions in photo/ electrocatalytic water splitting. Finally, the review looks forward to the development of advanced X-ray spectroscopies and their potential applications in catalytic water splitting reactions.

引用

页数：28

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