Aqueous Zn-CO2 batteries: a route towards sustainable energy storage

被引：8

作者：

Liu, Yanxiu ^{[1
]}

Chen, Junjie ^{[1
]}

Li, Weichen ^{[2
]}

Zhang, Yu ^{[1
]}

Fu, Xianwei ^{[2
]}

Li, Erling ^{[2
]}

Jin, Shangbin ^{[5
]}

Yang, Li-Ming ^{[6
]}

Tian, Zhihong ^{[2
]}

Antonietti, Markus ^{[3
]}

Liu, Tianxi ^{[4
]}

机构：

[1] East China Univ Sci & Technol, Sch Mech & Power Engn, Shanghai 200237, Peoples R China

[2] Henan Univ, Engn Res Ctr Nanomat, Kaifeng 475004, Peoples R China

[3] Max Planck Inst Colloids & Interfaces, Dept Colloid Chem, D-14476 Potsdam, Germany

[4] Jiangnan Univ, Sch Chem & Mat Engn, Key Lab Synthet & Biol Colloids, Minist Educ, Wuxi 214122, Peoples R China

[5] Xi An Jiao Tong Univ, Sch Chem Engn & Technol, 28 Xianning Rd, Xian 710049, Shaanxi, Peoples R China

[6] Huazhong Univ Sci & Technol, Sch Chem & Chem Engn, Wuhan 430074, Peoples R China

来源：

INDUSTRIAL CHEMISTRY & MATERIALS | 2024年 / 2卷 / 04期

基金：

中国国家自然科学基金; 上海市自然科学基金;

关键词：

ELECTROCATALYTIC CO2 REDUCTION; CARBON-DIOXIDE; DOPED CARBON; METAL; ELECTROREDUCTION; CATALYSTS; SITES; PERFORMANCE; GRAPHENE; CATHODE;

D O I：

10.1039/d4im00014e

中图分类号：

TQ [化学工业];

学科分类号：

0817 ;

摘要：

In recent years, the concept of rechargeable aqueous Zn-CO2 batteries has attracted extensive attention owing to their dual functionality of power supply and simultaneous conversion of CO2 into value-added chemicals or fuels. The state-of-the-art research has been mainly focused on the exploration of working mechanisms and catalytic cathodes but hardly applies an integrative view. Although numerous studies have proven the feasibility of rechargeable aqueous Zn-CO2 batteries, challenges remain including the low CO2 conversion efficiency, poor battery capacity, and low energy efficiency. This review systematically summarizes the working principles and devices, and the catalytic cathodes used for Zn-CO2 batteries. The challenges and prospects in this field are also elaborated, providing insightful guidance for the future development of rechargeable aqueous Zn-CO2 batteries with high performance.Keywords: Zn-CO2 battery; CO2 reduction reaction; Working mechanism; Electrocatalysts.

引用

页码：514 / 532

页数：19

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