Simultaneous control of time-dependent population transfer dynamics and wave-packet quantum interferences in Li2by shaped ultrafast pulses

被引：33

作者：

Ballard, Joshua B. ^{[1
,2
]}

Stauffer, Hans U. ^{[1
,2
]}

Mirowski, Elizabeth ^{[1
]}

Leone, Stephen R. ^{[1
,2
]}

机构：

[1] Dept. of Chemistry and Biochemistry, Natl. Inst. of Std. and Technology, University of Colorado, Boulder, CO 80309-0440, United States

[2] Lawrence Berkeley Natl. Laboratory, Department of Chemistry, University of California, Berkeley, CA 94720, United States

来源：

Physical Review A - Atomic, Molecular, and Optical Physics | 2002年 / 66卷 / 04期

关键词：

Algorithms - Bandwidth - Light interference - Mathematical models - Natural frequencies - Oscillations - Photoionization - Ultrashort pulses;

D O I：

10.1103/PhysRevA.66.043402

中图分类号：

学科分类号：

摘要：

Simultaneous control of time-dependent population transfer dynamics and wave-packet quantum interferences in Li2by shaped ultrafast pulses was discussed. It was shown that the optimal pulse shape for transient population transfer in the weak-field regime was characterized by nonresonant wavelengths. The degree to which the two states in the superposition can be independently controlled was quantified.

引用

页码：434021 / 434027