Study of the nitrogen fluorescence yield under different environmental conditions in alpha radioactivity telemetry technique

被引:0
|
作者
Wang, Quanxiao [1 ]
Li, Wanlin [1 ]
Pei, Xinfeng [1 ]
Song, Binghua [1 ]
Chen, Junliang [2 ,4 ]
Zhong, Yiqiang [2 ,3 ]
Li, Lianshun [2 ,4 ]
Wang, Jian [2 ]
Yang, Tinggui [2 ,3 ]
Si, Shuyao [2 ,3 ]
Fang, Kaihong [1 ,3 ]
机构
[1] Lanzhou Univ, Sch Nucl Sci & Technol, Lanzhou 730000, Peoples R China
[2] CNNC, 404 Co Ltd, Jiayuguan 735100, Peoples R China
[3] Key Lab Nucl Fuel Cycle Technol, Jiayuguan 735100, Peoples R China
[4] Chengdu Nucl Engn Design & Res Inst Co Ltd, CNNC 404, Chengdu 610000, Peoples R China
关键词
Fluorescence yield; alpha radioactivity telemetry technique; Energy dependence; Pressure dependence; Humidity dependence; Gas composition; AIR;
D O I
10.1016/j.nimb.2024.165605
中图分类号
TH7 [仪器、仪表];
学科分类号
0804 ; 080401 ; 081102 ;
摘要
alpha Decay in the nuclear fuel cycle poses significant hazards due to its strong ionizing capability, making effective detection essential. Conventional detection methods require time-consuming scanning or sampling, often unsuitable for extreme environments and increasing radiation risks. Alpha Radioactivity Telemetry Technology (ARTT), a non-contact alpha radiation detecting method via secondary nitrogen fluorescence detection, addresses the limitations of traditional methods and has gained significant attention in recent years. However, limited research on alpha-induced nitrogen fluorescence under varying conditions hampers environmental corrections and quantitative analysis, constraining applications of ARTT. This article examines the dependence of alpha-induced nitrogen fluorescence yield on energy, pressure, humidity, and nitrogen-oxygen ratio, presenting measurements for all major 2P system emission bands. The results indicate that (1) fluorescence yield remains unaffected by deposited energy or alpha-ray energy within 1.5-4 MeV, (2) yield dependence on pressure and humidity aligns with theoretical expectations, but deviates for nitrogen-oxygen ratios, and (3) temperature has minimal impact, with a 30 degrees C variation around 25 degrees C affecting fluorescence yield by less than 5 %. In contrast, at 1 atm pressure, the yield of air is several hundred times greater than at zero pressure. At 25 degrees C, the yield of dry air is 1.4 times that of air at 100 % RH. And the one of pure nitrogen is over ten times higher than the gas with 20 % nitrogen and 80 % oxygen. This work provides a data foundation for environmental corrections in ARTT applications.
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页数:9
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