Advances in inverted perovskite solar cells

被引：30

作者：

Zhang, Xin ^{[1
,2
,3
]}

Wu, Shengfan ^{[4
,5
,6
]}

Zhang, Hong ^{[1
,3
,7
]}

Jen, Alex K. Y. ^{[4
,5
,8
]}

Zhan, Yiqiang ^{[1
,2
,3
]}

Chu, Junhao ^{[1
,3
,7
]}

机构：

[1] Fudan Univ, State Key Lab Photovolta Sci & Technol, Shanghai, Peoples R China

[2] Fudan Univ, Ctr Micro Nano Syst, Sch Informat Sci & Technol SIST, Shanghai, Peoples R China

[3] Fudan Univ, Inst Optoelect, Shanghai Frontiers Sci Res Base Intelligent Optoel, Shanghai, Peoples R China

[4] City Univ Hong Kong, Dept Mat Sci & Engn, Hong Kong, Peoples R China

[5] City Univ Hong Kong, Hong Kong Inst Clean Energy, Hong Kong, Peoples R China

[6] Lingnan Univ, Sch Interdisciplinary Studies, Hong Kong, Peoples R China

[7] Fudan Univ, Dept Mat Sci, Shanghai, Peoples R China

[8] City Univ Hong Kong, Dept Chem, Hong Kong, Peoples R China

来源：

NATURE PHOTONICS | 2024年 / 18卷 / 12期

基金：

中国博士后科学基金; 中国国家自然科学基金;

关键词：

HIGH-PERFORMANCE; HOLE-TRANSPORT; INTERFACE PASSIVATION; HALIDE PEROVSKITES; CHARGE EXTRACTION; NICKEL-OXIDE; EFFICIENT; SILICON; CHALLENGES; LAYER;

D O I：

10.1038/s41566-024-01541-9

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

Considerable efforts are being made to advance inverted (p-i-n) perovskite solar cells (PSCs). Several passivation and insulation strategies have effectively been applied to reduce non-radiative recombination, a notorious issue for PSCs. Consequently, the performance of inverted PSCs has begun to rival those of regular (n-i-p) PSCs, with power conversion efficiency (PCE) values above 26%. The efficiency of tandem solar cells containing an inverted PSC as a subcell has also grown rapidly, reaching >33%. This Review discusses the origin of non-radiative recombinations in PSCs and recent progress in reducing them. We review how innovative device configurations, perovskite composition and interfacial engineering contribute to the high efficiency and long-term operational stability of inverted PSCs. We aim to provide readers with important insights into materials chemistry, physical processing and device configurations to further improve perovskite-based photovoltaics.

引用

页码：1243 / 1253

页数：11

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