Fabrication of flexible multifunctional graphene-based composite membrane with improved hydrophobicity and thermal conductivity characters for thermal management

被引:23
作者
Yang, Guoyan [1 ]
Yin, Zuozhu [1 ]
Deng, Yuanting [1 ]
Li, Zihao [1 ]
Chen, Yuhua [1 ]
Xiao, Wenbo [2 ]
Hong, Zhen [1 ]
Luo, Yidan [1 ]
Xie, Chan [1 ]
Xue, Mingshan [1 ]
机构
[1] Nanchang Hangkong Univ, Sch Mat Sci & Engn, 696 Fenghe South Rd, Nanchang 330063, Peoples R China
[2] Nanchang Hangkong Univ, Key Lab Nondestruct Testing, Minist Educ, Nanchang 330063, Peoples R China
基金
中国国家自然科学基金;
关键词
High temperature water vapor; Superhydrophobicity; High thermal conductivity; Graphene; Composite coatings;
D O I
10.1016/j.colsurfa.2024.135494
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The lifetime of electronic devices in complex environments is affected by the impact of high temperature water vapor on their performance. Equipping electronic devices with superhydrophobic properties and improved thermal conductivity will be the strategy of the future. In this paper, a surface material with high thermal conductivity and superhydrophobic properties is explored to address the problem of electronic device failure caused by heat and water vapor. To solve this problem, anti-temperature superhydrophobicity can be obtained by spraying alumina/nano-silicon carbide/thermoplastic elastomer composite powder (Al2O3/nano-SiC/SEBS) modified with 1 H,1 H,2 H,2H-perfluorooctyltriethoxysilane (POTS) on graphene membranes. A spherical Al2O3/nano-SiC composite superhydrophobic coating (ASS-GM) was formed on the surface of graphene-based composite membranes by spraying method. The results showed that the optimal ratio was m(Al2O3): m(SiC) = 8:1, and the static water contact angle of the coating was 162 +/- 2.5 degrees, and the surface energy was reduced. The ASS-GM significantly improves the thermal conductivity and superhydrophobicity of graphene-based composite membranes, achieving a double improvement in performance. The coating also offers excellent self-cleaning and antifouling properties compared to other materials. The ASS-GM is able to maintain a certain hydrophobicity angle (156 +/- 1.5 degrees) in harsh environments. This work provides practical applications for electronic coatings, which are important for improving the overall reliability and durability of electronic products.
引用
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页数:12
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