Nanoarchitectonics of MoS2 petals with 0D@2D carbon derivatives for integrated photocapacitor application

被引:3
作者
Arjunkumar, B. [1 ]
Keerthana, T. [1 ]
Ramalingam, Gopal [1 ]
Vetrivelan, V. [2 ]
Ragupathi, C. [3 ]
Mangalaraja, R. V. [4 ,5 ]
Alam, Mohammed Mujahid [6 ,7 ]
Anbukumaran, S. K. [8 ]
机构
[1] Alagappa Univ, Dept Nanosci & Technol, Quantum Mat Res Lab QMRL, Karaikkudi 630003, Tamil Nadu, India
[2] Govt Coll Engn, Dept Phys, Tiruchirappalli 620012, Tamil Nadu, India
[3] Sriram Coll Arts & Sci, Dept Chem, Tiruvallur 602024, India
[4] Univ Adolfo Ibaenez, Fac Engn & Sci, Diagonal Torres 2640, Santiago 7941169, Chile
[5] Univ Arturo Prat, Vicerrectoria Invest Innovac, Ave Arturo Prat 2120, Iquique 1110939, Chile
[6] King Khalid Univ, Coll Sci, Dept Chem, Abha 61413, Saudi Arabia
[7] King Khalid Univ, Res Ctr Adv Mat Sci RCAMS, Abha 61413, Saudi Arabia
[8] Saveetha Univ, Saveetha Inst Med & Tech Sci, Ctr Global Hlth Res, Chennai 602105, India
关键词
MoSS nanopetals; DSSC; Supercapcitor; Photocapacitor; HYDROTHERMAL SYNTHESIS; HIGH-EFFICIENCY; NICKEL-OXIDE; SOLAR; SUPERCAPACITOR; PERFORMANCE; DOTS; NANOSPHERES; NANOSHEETS; DEVICE;
D O I
10.1016/j.jallcom.2024.177622
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Photocapacitors are a breakthrough in energy storage and generation, storing and generating solar energy in several ways. Sustainable technology and satisfying the energy needs of a rapidly changing planet depend on their progress. A hydrothermal technique was used to synthesize carbon quantum dots-ornamental MoSS nanopetals on reduced graphene oxide (rGO). XRD, Raman, and XPS validated the hybrid nanomaterial's phase purity, composition, and oxidation state. Morphological research showed MoSS nanopetals producing a flowerlike structure with evenly dispersed carbon quantum dots on a thin, twisted sheet. As a counter electrode in dye-sensitized solar cells (DSSCs), this hybrid material increased efficiency by 6.7 % and photovoltaic characteristics. An asymmetric supercapacitor made from the hybrid material and activated carbon had 166.6 F/g specific capacitance at 5 mV/s and 81.5 % capacitance retention after 5000 charge-discharge cycles. The combined photocapacitor device, combining DSSC and supercapacitor, obtained 4.4 % overall efficiency and 34 % storage efficiency. The MoSS nanopetals-based electrode shows promise for photocapacitor applications, potentially improving future flexible and wearable technologies.
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页数:14
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