Influence of regularization matrix on inversion of bimodal dynamic light scattering data

被引:0
作者
Liu, Wei [1 ]
Wang, Yajing [1 ]
Chen, Wengang [1 ]
Ma, Lixiu [1 ]
Shen, Jin [1 ]
机构
[1] School of Electrical and Electronic Engineering, Shandong University of Technology, Zibo, 255049, Shandong
来源
Zhongguo Jiguang/Chinese Journal of Lasers | 2015年 / 42卷 / 09期
关键词
Bimodal distribution particles; Dynamic light scattering; Particle; Scattering; size inversion; Tikhonov regularization;
D O I
10.3788/CJL201542.0908003
中图分类号
学科分类号
摘要
The inversion of bimodal dynamic light scattering data is very difficult. Tikhonov regularization method is the often used inversion algorithm, however, the influence of different regularization matrices on the inversion is not clear yet. Two bimodal particle size distributions with 6 levels of noise are inverted by using identity matrix L1, first order difference matrix L2 and second order differential matrix L3. Simulation data shows that the bimodal resolution decrease with the increase of noise level. The anti-interference ability of the algorithm is stronger when the components of bimodal distribution are closer. Under the same noise level, the bimodal resolution of matrix L3 is of the best, while the error of inversion is minimum; correspondingly the bimodal resolution of matrix L1 is of the worst, while the error of inversion is maximum. The matrix L3 can distinguish the smallest peak value size ratio, while matrix L1 can only distinguish the biggest peak value size ratio. Under the same noise level, peak value size ratio is bigger and the bimodal resolution is stronger. Therefore, matrix L3 should be used in order to get the correct inversion result by inverting the noisy scattering data. Finally, the inversion of experimental particles confirms this conclusion. �, 2015, Science Press. All right reserved.
引用
收藏
页数:10
相关论文
共 18 条
  • [1] Liu W., Wang Y., Shen J., Optimal fitting cumulants method for dynamic light scattering, Acta Optica Sinica, 33, 12, (2013)
  • [2] Dou Z., Wang Y., Shen J., Et al., A hybrid non-negative constraint inversion of dynamic light scattering based on truncated singular value decomposition, Chinese J Lasers, 40, 6, (2013)
  • [3] Wang Z., Cai X., Xu C., Et al., Nanoparticle sizing by image processing with dynamic light scattering, Acta Optica Sinica, 34, 1, (2014)
  • [4] Provencher S.W., CONTIN: A general purpose constrained regularization program for inverting noisy linear algebraic and integral equations, Comput Phy Commun, 27, 3, pp. 229-242, (1982)
  • [5] Mcwhirter J.G., Pike E.R., On the numerical inversion of the Laplace transform and similar Fredholm integral equations of the first kind, Phys A: Math Gen, 11, 9, pp. 1729-1745, (1978)
  • [6] Dahneke B.E., Measurement of Suspended Partieles by Quasi-Elastie Light Scattering, (1983)
  • [7] Sun Y.F., Walker J.G., Maximum likelihood data inversion for photon correlation spectroscopy, Meas Sci Technol, 19, 11, (2008)
  • [8] Morrison I.D., Grabowski E.F., Herb C.A., Improved techniques for particle size determination by quasi-elastic light scattering, Langmuir, 1, 4, pp. 496-501, (1985)
  • [9] Han Q., Shen J., Sun X., Et al., A posterior choice strategies of the tikhonov regularization parameter in the inverse algorithm of the photon correlation spectroscopy particle sizing techniques, Acta Photonica Sinica, 38, 11, pp. 2917-2926, (2009)
  • [10] Zhu X.J., Shen J., Liu W., Et al., Nonnegative least-squares truncated singular value decomposition to particle size distribution inversion from dynamic light scattering data, Appl Opt, 49, 34, pp. 6591-6596, (2010)