Experimental investigation on the effect of channel geometry on performance heterogeneity in hydrogen PEM fuel cell

被引:1
作者
Casadei, Delio [1 ]
Verducci, Francesco [1 ]
Grimaldi, Amedeo [1 ]
Croci, Diego [2 ]
Palmieri, Alessandro [2 ]
Bianchi, Roberto [2 ]
Picciotti, Gianmario [2 ]
Casalegno, Andrea [1 ]
Baricci, Andrea [1 ]
机构
[1] Politecn Milan, Energy Dept, Via Lambruschini 4a, I-20156 Milan, Italy
[2] Eldor Corp SpA, Via Don Paolo Berra 18, I-22030 Orsenigo, CO, Italy
关键词
Polymer electrolyte membrane fuel cell; Flow field; Heterogeneity; Channel; Electrical contact; Transport resistance; OXYGEN-TRANSPORT RESISTANCE; GAS-DIFFUSION LAYER; FLOW-FIELDS; WATER SATURATION; CATALYST LAYER; BIPOLAR PLATES; IMPACT; POWER;
D O I
10.1016/j.ijhydene.2024.08.515
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Straight parallel graphite-based flow fields are experimentally assessed to evaluate the effect of geometrical parameters on the performance of polymer electrolyte membrane fuel cell. A 1+1D fuel cell model is exploited to evaluate the local operating conditions occurring along various positions of the flow field channel for different load requirements. The estimated operating conditions are implemented in a zero-gradient hardware to perform a broad experimental campaign, conducting tests under controlled and uniform operating conditions. The achieved experimental results depict the impact of the flow field geometry along different positions of the flow field channel under real operating conditions, identifying the individual contributions of the geometric parameters on water transport, oxygen transport and electrical resistance. The proposed methodology provides detailed information on the local operation of a large-area bipolar plate using a small-area sample, demonstrating the effect of rib and channel geometrical parameters on real-world operation of a PEMFC.
引用
收藏
页码:1299 / 1315
页数:17
相关论文
共 72 条
  • [11] Song Y., Zhang C., Ling C.Y., Han M., Yong R.Y., Sun D., Et al., Review on current research of materials, fabrication and application for bipolar plate in proton exchange membrane fuel cell, Int J Hydrogen Energy, 45, pp. 29832-29847, (2020)
  • [12] Bi F., Yi P., Zhou T., Peng L., Lai X., Effects of Al incorporation on the interfacial conductivity and corrosion resistance of CrN film on SS316L as bipolar plates for proton exchange membrane fuel cells, Int J Hydrogen Energy, 40, pp. 9790-9802, (2015)
  • [13] Wilberforce T., Ijaodola O., Ogungbemi E., Khatib F.N., Leslie T., El-Hassan Z., Et al., Technical evaluation of proton exchange membrane (PEM) fuel cell performance – a review of the effects of bipolar plates coating, Renew Sustain Energy Rev, 113, (2019)
  • [14] Gao X., Chen J., Xu R., Zhen Z., Zeng X., Chen X., Et al., Research progress and prospect of the materials of bipolar plates for proton exchange membrane fuel cells (PEMFCs), Int J Hydrogen Energy, 50, pp. 711-743, (2024)
  • [15] Thapa S., Ganesh V., Agarwal H., Sahu A.K., Performance evaluation of cathode channels with different cross-sections for open-cathode polymer electrolyte membrane fuel cell stack, J Power Sources, 603, (2024)
  • [16] Wang X.R., Ma Y., Gao J., Li T., Jiang G.Z., Sun Z.Y., Review on water management methods for proton exchange membrane fuel cells, Int J Hydrogen Energy, 46, pp. 12206-12229, (2021)
  • [17] Benkovic D., Fink C., Iranzo A., Qualitative and quantitative determination of liquid water distribution in a PEM fuel cell, Int J Hydrogen Energy, 52, pp. 1360-1370, (2024)
  • [18] Gwak G., Lee J., Ghasemi M., Choi J., Lee S.W., Jang S.S., Et al., Analyzing oxygen transport resistance and Pt particle growth effect in the cathode catalyst layer of polymer electrolyte fuel cells, Int J Hydrogen Energy, 45, pp. 13414-13427, (2020)
  • [19] Ding Q., Zhu K.Q., Xu J.H., Zhang B.X., Yang Y.R., Yang C., Et al., Evaluation criterion of flow fields in PEM fuel cells based on entropy generation analysis, Int J Hydrogen Energy, 48, pp. 2328-2340, (2023)
  • [20] Colombo E., Baricci A., Bisello A., Guetaz L., Casalegno A., PEMFC performance decay during real-world automotive operation: evincing degradation mechanisms and heterogeneity of ageing, J Power Sources, 553, (2023)