Research progress on the direct regeneration technology for cathode materials from spent lithium-ion batteries

被引：0

作者：

Li, Hongyan ^{[1
]}

Xie, Shuhan ^{[1
]}

Zhang, Yanru ^{[1
]}

Wang, Yongjing ^{[1
]}

Wang, Yonghao ^{[1
]}

Lyu, Yuancai ^{[1
]}

Lin, Chunxiang ^{[1
]}

Li, Xiaojuan ^{[1
]}

机构：

[1] College of Environment & Safety Engineering, Fuzhou University, Fujian, Fuzhou

来源：

Huagong Jinzhan/Chemical Industry and Engineering Progress | 2024年 / 43卷 / 09期

关键词：

cathode materials; direct regeneration; lithium-ion batteries (LIBs); recycling;

D O I：

10.16085/j.issn.1000-6613.2023-1356

中图分类号：

学科分类号：

摘要：

With the rapid growth of the demand for lithium-ion battery (LIBs), a large number of waste LIBs will be produced. If not disposed of properly, it will bring serious environmental pollution problems. The cathode materials of spent LIBs contain a large number of rare valuable metals, and the recovery of these metals will produce both environmental and economic benefits. Compared with the traditional separation, purification and recovery technologies of metal components from cathode materials, the strategy of direct regeneration of cathode materials has attracted much attention due to its advantages of simple process, low energy consumption, short recycling cycle and high added value of products. Six direct regeneration technologies for cathode materials from spent LIBs such as coprecipitation method, sol-gel method, solid phase sintering method, hydrothermal method, ion thermal/molten salt method and electrochemical repair method were reviewed and their advantages and disadvantages were also summarized. Among them, coprecipitation method and sol-gel method had some limitations in industrial application because of their relatively complex steps, high equipment requirements and reagent cost. Solid phase sintering method, hydrothermal method, ion thermal/molten salt method and electrochemical repair method had great opportunities for development because of their convenience and economy. In addition, the prospect and development trend of direct recycling of cathode materials from spent LIBs were prospected in order to provide reference for the research in the field of spent LIBs recycling. © 2024 Chemical Industry Press Co., Ltd.. All rights reserved.

引用

页码：5207 / 5216

页数：9

共 63 条

[1] ETACHERI Vinodkumar, MAROM Rotem, ELAZARI Ran, Et al., Challenges in the development of advanced Li-ion batteries: A review, Energy & Environmental Science, 4, 9, pp. 3243-3262, (2011)
[2] XU Panpan, YANG Zhenzhen, YU Xiaolu, Et al., Design and optimization of the direct recycling of spent Li-ion battery cathode materials, ACS Sustainable Chemistry & Engineering, 9, 12, pp. 4543-4553, (2021)
[3] MALLICK Sourav, PATEL Arjun, SUN Xiaoguang, Et al., Low-cobalt active cathode materials for high-performance lithium-ion batteries: Synthesis and performance enhancement methods, Journal of Materials Chemistry A, 11, 8, pp. 3789-3821, (2023)
[4] ZHU Xiangdong, XIAO Jin, MAO Qiuyun, Et al., A promising regeneration of waste carbon residue from spent Lithium-ion batteries via low-temperature fluorination roasting and water leaching, Chemical Engineering Journal, 430, (2022)
[5] MEEGODA Jay N, MALLADI Sarvagna, ZAYAS Isabel C., End-of-life management of electric vehicle lithium-ion batteries in the United States, Clean Technologies, 4, 4, pp. 1162-1174, (2022)
[6] HE Kai, ZHANG Zhiyuan, ZHANG Fushen, A green process for phosphorus recovery from spent LiFePO4 batteries by transformation of delithiated LiFePO4 crystal into NaFeS2, Journal of Hazardous Materials, 395, (2020)
[7] ZHAO Yanlan, YUAN Xingzhong, JIANG Longbo, Et al., Regeneration and reutilization of cathode materials from spent lithium-ion batteries, Chemical Engineering Journal, 383, (2020)
[8] NEUMANN Jonas, PETRANIKOVA Martina, MEEUS Marcel, Et al., Recycling of lithium-ion batteries—Current state of the art, circular economy, and next generation recycling, Advanced Energy Materials, 12, 17, (2022)
[9] YANG Yue, OKONKWO Emenike G, HUANG Guoyong, Et al., On the sustainability of lithium ion battery industry—A review and perspective, Energy Storage Materials, 36, pp. 186-212, (2021)
[10] LAROUCHE Francois, TEDJAR Farouk, AMOUZEGAR Kamyab, Et al., Progress and status of hydrometallurgical and direct recycling of Li-ion batteries and beyond, Materials, 13, 3, (2020)

← 1 2 3 4 5 6 7 →