An all solid waste CO2 sequestration material consist of multiple calcium silicate clinkers by carbide slag, copper tailing and red mud: Clinker crystal transformation and carbonation hardening properties

被引:1
|
作者
Wang, Shengmin [1 ,2 ]
Zou, Fubing [3 ,4 ]
Luo, Hongyun [3 ,4 ]
机构
[1] Wuhan Text Univ, State Key Lab New Text Mat & Adv Proc Technol, Wuhan 430070, Peoples R China
[2] Wuhan Text Univ, Sch Accountancy, Wuhan 430070, Peoples R China
[3] Nanchang Univ, Sch Infrastruct Engn, Nanchang 330031, Peoples R China
[4] Nanchang Univ, Chongqing Res Inst, Chongqing 402660, Peoples R China
基金
中国国家自然科学基金;
关键词
Red mud; Calcium silicate clinkers; Crystal regulator; Carbonation and hardening; Microstructure; CO2 sequestration materials; STRENGTH;
D O I
10.1016/j.conbuildmat.2024.138534
中图分类号
TU [建筑科学];
学科分类号
0813 ;
摘要
In this study, a CO2 2 sequestration material was obtained by all components solid wastes, i.e., carbide slag and copper tailing based on red mud (RM) as crystal regulator after a sintering and carbonation process. With the increasing dosage of RM, the mineral compositions of generated RM-modified clinkers were mainly gamma-C2S 2 S (i.e., around 80 %) at low dosage RM (i.e., 3.0 %), and was gradually increased content of beta-C2S 2 S (beta-dicalcium silicate), C3S 3 S (tricalcium silicate) and C2AS 2 AS (gehlenite) at high dosage RM (i.e., from 3.0 % to 10.0 %). Moreover, the compressive strength of various carbonated compacts made by RM-modified clinkers after CO2 2 curing were shows firstly increased and then decreased with a RM dosage inflection of 5.0 %. This compressive strength results should be attributed to their carbonation activity, i.e., higher carbonation activity, higher compressive strength. The obvious carbonation activity difference of various RM-modified clinkers were not simply depends on their only gamma-C2S 2 S content, only beta-C2S 2 S content, only C3S 3 S content or the sum of calcium silicate minerals, but more closely relate to their combined effect. This work provides a new utilization strategy of RM as crystal regulator according to its high alkaline and high Fe content composition characteristic for obtaining a CO2 2 sequestration materials. And also laid a new insight for a synergistic CO2 2 sequestration by multiple calcium silicate clinkers in the future.
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页数:17
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