Construction of dual Z-scheme Ag3VO4–BiVO4/InVO4 photocatalysts using vanadium source from spent catalysts for contaminated water treatment and bacterial inactivation

被引:1
作者
Lee K.-C. [1 ,2 ]
Hsu S.-C. [3 ]
Huang J.-H. [4 ]
Wang K.-S. [5 ]
Pang W.K. [6 ]
Hu C.-W. [7 ]
Jiang Y.-J. [8 ]
Cho E.-C. [8 ]
Weng H.C. [9 ]
Liu T.-Y. [5 ,10 ,11 ]
机构
[1] Department of Science Education, National Taipei University of Education, No. 134, Sec. 2, Heping E. Road, Da-an District, Taipei City
[2] PhD Program in Medical Neuroscience, College of Medical Science and Technology, Taipei Medical University, 250 Wuxing Street, Taipei City
[3] Department of Chemical and Materials Engineering, Tamkang University, No. 151, Yingzhuan Road, Tamsui District, New Taipei City
[4] Department of Green Material Technology, Green Technology Research Institute, CPC Corporation, No.2, Zuonan Rd., Nanzi District, Kaohsiung City
[5] Department of Materials Engineering, Ming Chi University of Technology, New Taipei City
[6] Faculty of Engineering, Institute for Superconducting & Electronic Materials, University of Wollongong, Wollongong, NSW
[7] National Synchrotron Radiation Research Center, 101 Hsin-Ann Road, Hsinchu Science Park, Hsinchu
[8] School of Pharmacy, College of Pharmacy, Taipei Medical University, 250 Wuxing Street, Taipei City
[9] Department of Mechanical Engineering, Chung Yuan Christian University, No. 200, Chungpei Road, Chungli District, Taoyuan City
[10] Department of Chemical Engineering and Materials Science, Yuan Ze University, Taoyuan City
[11] College of Engineering & Center for Sustainability and Energy Technologies, Chang Gung University, Taoyuan
关键词
Ag[!sub]3[!/sub]VO[!sub]4[!/sub]/BiVO[!sub]4[!/sub]/InVO[!sub]4[!/sub; Bacterial inactivation; Photocatalyst; Vanadium recovery; Z-scheme;
D O I
10.1016/j.chemosphere.2024.142746
中图分类号
学科分类号
摘要
Vanadate-based photocatalysts have recently attracted substantial attention owing to their outstanding photocatalytic activity for degrading organic pollutants and generating energy via photocatalytic processes. However, the relatively high price of vanadium has hindered the development of vanadate-based photocatalysts for various applications. Spent catalysts obtained from oil refineries typically contain a significant quantity of vanadium, making them valuable for recovery and utilization as precursors for the production of high-value-added photocatalysts. In this study, we transformed the V present in spent catalysts produced by the petrochemical industry into ternary vanadate-based photocatalysts [BiVO4/InVO4/Ag3VO4 (BVO/IVO/AVO, respectively)] designed for water remediation. The ternary composites revealed an enhanced photocatalytic capability, which was 1.42 and 5.1 times higher than those of the binary BVO/IVO and pristine AVO due to the facilitated charge separation. The ternary photocatalysts not only effectively treated wastewater containing various organic dyes, such as methylene blue (MB), rhodamine 6G (R6G), and brilliant green (BG), but also exhibited remarkable photocatalytic performance in the degradation of antibiotics, reduction of Cr(VI), and bacterial inactivation. This paper proposes a feasible route for recycling industrial waste as a source of vanadium to produce highly efficient vanadate-based photocatalysts. © 2024 Elsevier Ltd
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