Atmospheric pressure dielectric barrier discharge plasma for in-situ water treatment using a bubbling reactor

被引:2
作者
Tang, Xin [1 ]
Ferraz Jr, Antonio D. N. [2 ]
Karu, Kersti [3 ]
Campos, Luiza C. [2 ]
Kim, Minkwan [1 ]
机构
[1] Univ Southampton, Dept Aeronaut & Astronaut Engn, Southampton SO16 7QF, England
[2] UCL, Ctr Urban Sustainabil & Resilience, Dept Civil Environm & Geomat Engn, Gower St, London WC1E 6BT, England
[3] UCL, Dept Chem, UCL Chem Mass Spectrometry Facil, London WC1E 6BT, England
关键词
In-situ resource utilization (ISRU); Non-thermal plasma; Dielectric barrier discharge; Sulfamethoxazole degradation; E. coli K12 inactivation; ADVANCED OXIDATION PROCESSES; ESCHERICHIA-COLI; NONTHERMAL PLASMA; WASTE-WATER; SULFADIAZINE ANTIBIOTICS; RISK-ASSESSMENT; DEGRADATION; PHARMACEUTICALS; INACTIVATION; REMOVAL;
D O I
10.1016/j.jenvman.2024.122574
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Non-thermal plasma has been an emerging technology for water treatment for decades. In this study, we have designed and fabricated a bubbling plasma batch reactor using an atmospheric pressure dielectric barrier discharge with a hydrophobic porous membrane. The reactor performance is assessed for purifying synthetic contaminated water samples containing chemical contaminant sulfamethoxazole (SMX), a widely used antibiotic, and biological contaminant E. coli K12. The SMX decontamination tests indicate that the degradation process is not first-order and the reaction rate dwindle with increasing initial concentration. The yield at 50% removal achieves its highest value of 8.12 g/kWh for 50 mg/L SMX sample. For inactivation of E. coli K12 tests, the inactivation process is also not first-order, and the pathogen is completely inactivated for 10(2) CFU/mL and 10(4) CFU/mL cases after 10 min and 45 min of plasma treatment, respectively. For the 10(8) CFU/mL sample, a 5-log reduction is achieved after 60 min of treatment. The developed plasma reactor can achieve fast deployment in point of use, low cost for manufacturing, and simple for maintenance. Moreover, it can be used for in-situ water purification in future long duration crewed space missions as well as tackling with water pollution issues on our planet.
引用
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页数:10
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