Facile synthesis, characterization and optical properties of Ag2WO4 incorporated g-C3N4 hybrid composites for H2 production

被引:0
作者
Kavitha, T. [1 ]
Renukadevi, S. [1 ]
Veerasamy, R. [2 ,3 ]
机构
[1] KSR Coll Engn, Dept Phys, Tiruchengode 637215, Tamilnadu, India
[2] Karpagam Acad Higher Educ, Dept Chem, Coimbatore 641064, Tamilnadu, India
[3] KSR Coll Engn, Dept Chem, Tiruchengode 637215, Tamilnadu, India
关键词
GRAPHITIC CARBON NITRIDE; VISIBLE-LIGHT; PHOTOCATALYTIC ACTIVITY; NANOSHEETS; HETEROJUNCTION; NANOPARTICLES; NANOCOMPOSITE; DISINFECTION; PERFORMANCE; REMOVAL;
D O I
10.1007/s10854-024-13569-2
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
The hydrothermal approach was used to synthesise a composite photocatalyst of Ag2WO4/g-C3N4. This photocatalyst proved effective in preventing Escherichia coli (E. coli) when exposed to visible light. Imaging microscopy, transmission electron microscopy (TEM), X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FTIR), N-2 adsorption-desorption analysis, UV-Vis diffuse reflectance spectra (DRS), and photoluminescence (PL) were among the many methods used to comprehensively characterize the photocatalysts' physicochemical characteristics. In comparison to pure g-C3N4 and Ag2WO4 under visible light, the produced photocatalysts demonstrated significantly improved photocatalytic cleaning efficiency. In addition, under visible light irradiation for 60 min, a mixture of 5 percent Ag2WO4 and 100 milligrammes of g-C3N4 was able to entirely kill many live bacteria. The ideal mass ratio for this combination was 5 weight percent. By working in tandem, g-C3N4 and Ag2WO4 increase the separation rate of photogenerated electron-hole pairs and ensure that Ag2WO4 particles are evenly distributed over the g-C3N4 surface, leading to a high disinfection efficiency. These hybrids outperform pure g-C3N4 in the visible range when it comes to the efficiency of hydrogen evolution (3761.1 mu mol h(-1) g(-1)). A higher degree of photocatalytic activity may be achieved in the composite Ag2WO4/g-C3N4 photocatalyst through boosting the spacing of charge carriers produced by photons in the two photocatalysts.
引用
收藏
页数:14
相关论文
共 50 条
  • [41] The facile synthesis of mesoporous g-C3N4 with highly enhanced photocatalytic H2 evolution performance
    He, Fang
    Chen, Gang
    Zhou, Yansong
    Yu, Yaoguang
    Zheng, Yi
    Hao, Sue
    CHEMICAL COMMUNICATIONS, 2015, 51 (90) : 16244 - 16246
  • [42] High efficiency for H2 evolution and NO removal over the Ag nanoparticles bridged g-C3N4 and WS2 heterojunction photocatalysts
    Ma, Yongning
    Li, Juan
    Liu, Enzhou
    Wan, Jun
    Hu, Xiaoyun
    Fan, Jun
    APPLIED CATALYSIS B-ENVIRONMENTAL, 2017, 219 : 467 - 478
  • [43] Improved photocatalytic H2 production assisted by aqueous glucose biomass by oxidized g-C3N4
    Speltini, Andrea
    Scalabrini, Andrea
    Maraschi, Federica
    Sturini, Michela
    Pisanu, Ambra
    Malavasi, Lorenzo
    Profumo, Antonella
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2018, 43 (32) : 14925 - 14933
  • [44] Facile one-pot pyrolysis preparation of SnO2/g-C3N4 composites for improved photocatalytic H2 production
    Cai, Chongze
    Wang, Zihao
    Shi, Jinwen
    Zhang, Yazhou
    Mao, Liuhao
    Chen, Feng
    Wang, Tianhao
    Chen, Yubin
    JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY, 2022, 97 (10) : 2921 - 2931
  • [45] g-C3N4 Nanosheet Nanoarchitectonics: H2 Generation and CO2 Reduction
    Zhang, Xiao
    Yang, Ping
    CHEMNANOMAT, 2023, 9 (06)
  • [46] One-step synthesis of C quantum dots/C doped g-C3N4 photocatalysts for visible-light-driven H2 production from water splitting
    Cao, Jian
    Jin, Xiaoli
    Ma, Zhaoyu
    Wang, Huiqing
    Xu, Yixue
    Guo, Yuwei
    Xie, Haiquan
    Zhang, Junying
    JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2022, 55 (44)
  • [47] Synthesis of g-C3N4/WO3-carbon microsphere composites for photocatalytic hydrogen production
    Sun, Meng
    Zhou, Yunlong
    Yu, Teng
    Wang, Jian
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2022, 47 (18) : 10261 - 10276
  • [48] Fabrication and photocatalytic activity enhanced mechanism of direct Z-scheme g-C3N4/Ag2WO4 photocatalyst
    Zhu, Bicheng
    Xia, Pengfei
    Li, Yao
    Ho, Wingkei
    Yu, Jiaguo
    APPLIED SURFACE SCIENCE, 2017, 391 : 175 - 183
  • [49] Methylene Blue Incorporated Donor-Acceptor g-C3N4 Nanosheet Photocatalyst for H2 Production
    Yin, Fangxin
    Qin, Pinquan
    Xu, Jingsan
    Cao, Shaowen
    ACTA PHYSICO-CHIMICA SINICA, 2023, 39 (11)
  • [50] Construction of hybrid 2D g-C3N4/BiVO4 photocatalyst decorated with RGO for enhancing the H2 production and photocatalytic degradation of antibiotics
    Kavitha., T.
    Rojviroon, Orawan
    Rajendran, Ranjith
    Rojviroon, Thammasak
    JOURNAL OF POROUS MATERIALS, 2025,