Characteristics and Source Apportionment of Atmospheric Fine Particles in Langfang in Autumn and Winter

被引：0

作者：

Zhu S.-Z. ^{[1
]}

Tong J. ^{[1
]}

Bao F. ^{[1
]}

Sun H. ^{[1
]}

机构：

[1] Langfang Municipal Ecology and Environment Bureau, Langfang

来源：

Huanjing Kexue/Environmental Science | 2023年 / 44卷 / 01期

关键词：

atmospheric particulate matter; chemical composition; Langfang; mass closure; source apportionment;

D O I：

10.13227/j.hjkx.202112128

中图分类号：

学科分类号：

摘要：

In this study, we report observations of various chemical species in PM2.5 samples that were collected between November 25, 2019 and March 31, 2020 in the northern, urban, and southern areas of Langfang, among which the concentrations of PM2. 5 followed the order of southern > urban > northern. The abundance and chemical compositions of the particles in this study were temporally and spatially variable, with major contributions from organic matter (25. 4%), nitrate (21. 5%), sulfate (11. 0%), ammonium (13. 5%), and crustal matter (13. 7%). The contributions of nitrate, sulfate, and ammonium were higher in the urban site compared with that in the southern and northern sites. On the contrary, organic matter and crustal matter exhibited much higher values in the southern and northern sites. In addition, the contributions of organic matter to the particle mass decreased from 27. 3% to 23. 0%, and the total contributions of sulfate, nitrate, and ammonium ions increased from 38. 7% to 51.3% between clean and haze days, respectively. Source apportionment using positive matrix factorization showed five PM2.5 sources: secondary inorganic aerosol (41.9%), traffic emissions (19. 9%), coal combustion (12.7%), industrial pollution (9. 1%), and mineral dust (9.3%). The contributions of the first two factors followed the order of urban > northern > southern, whereas the contributions of the last three factors followed the order of southern > northern > urban. Further, the contributions of secondary inorganic aerosol, traffic emissions, and coal combustion were higher on haze days, whereas the contributions of industrial pollution and mineral dust were higher on clean days. © 2023 Science Press. All rights reserved.

引用

页码：20 / 29

页数：9

共 45 条

[1] Zhang Y H, Song Y Y, Chen Y J, Et al., Discovery of emerging sulfur-containing PAHs in PM2. 5 : contamination profiles and potential health risks, Journal of Hazardous Materials, 416, (2021)
[2] Zhang Y Q., All-cause mortality risk and attributable deaths associated with long-term exposure to ambient PM2. 5 in Chinese adults[ J], Environmental Science & Technology, 55, 9, pp. 6116-6127, (2021)
[3] Huang R J, Zhang Y L, Bozzetti C, Et al., High secondary aerosol contribution to particulate pollution during haze events in China, Nature, 514, 7521, pp. 218-222, (2014)
[4] Cao Y, Wang M H, Rosenfeld D, Et al., Strong aerosol effects on cloud amount based on long-term satellite observations over the east coast of the United States [ J ], Geophysical Research Letters, 48, 6, (2021)
[5] Wang Y H, Gao W K, Wang S, Et al., Contrasting trends of PM2. 5 and surface-ozone concentrations in China from 2013 to 2017, National Science Review, 7, 8, pp. 1331-1339, (2020)
[6] Wang Y S, Li W J, Gao W K, Et al., Trends in particulate matter and its chemical compositions in China from 2013- 2017, Science China Earth Sciences, 62, 12, pp. 1857-1871, (2019)
[7] Lei L, Zhou W, Chen C, Et al., Long-term characterization of aerosol chemistry in cold season from 2013 to 2020 in Beijing, China, Environmental Pollution, 268, (2020)
[8] Shi Y P, Chu Y X, Duan J C, Et al., Identification rule and algorithm for regional heavy air pollution processes, Environmental Monitoring in China, 37, 4, pp. 32-39, (2021)
[9] Zheng M, Salmon L G, Schauer J J, Et al., Seasonal trends in PM2. 5 source contributions in Beijing, China, Atmospheric Environment, 39, 22, pp. 3967-3976, (2005)
[10] Qiao T, Zhao M F, Xiu G L, Et al., Simultaneous monitoring and compositions analysis of PM1 and PM2. 5 in Shanghai: implications for characterization of haze pollution and source apportionment, Science of the Total Environment, 557-558, pp. 386-394, (2016)

← 1 2 3 4 5 →