Review Advances in light-enhanced biological/artificial hybrid systems

被引:0
作者
Bo, Chunling [1 ,2 ]
Liu, Jing [1 ]
Chen, Xiaobo [3 ]
Piao, Lingyu [1 ,4 ]
机构
[1] Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China
[2] Univ Chinese Acad Sci, Ctr Mat Sci & Optoelect Engn, Beijing 100049, Peoples R China
[3] Univ Missouri, Dept Chem, Kansas City, MO 64110 USA
[4] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
基金
中国国家自然科学基金;
关键词
Biological/artificial photocatalytic sys-tems integrate the high solar absorptionof semiconductors and high selectivityof biocatalysts for promising water split-ting; CO2conversion; and N2reductionreactions; Meticulous construction of the systemswith suitable components and efficientelectron transfer between componentsare crucial to gain high reaction efficiencyand stability; Future better understanding of electrontransfer and metabolic pathways withinthe systems will advance both the effi-ciency and selectivity of photosynthesisprocesses; HYDROGEN-PRODUCTION; ESCHERICHIA-COLI; CARBON-DIOXIDE; H-2; PRODUCTION; SOLAR; CATALYSIS; CO2; EFFICIENCY; REDUCTION; EVOLUTION;
D O I
10.1016/j.trechm.2024.08.006
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Converting small molecules such as H2O, 2 O, CO2, 2, and N2 2 into high value-added products not only facilitates green energy production but also contributes to global material circulation. While it remains a challenge to achieve high activity and selectivity simultaneously using artificial photocatalytic systems, biological/artificial hybrid systems, which combine the high-efficiency utilization of light energy of light-sensitive materials with the remarkable selectivity of biocatalysts, have shown promising trends to overcome such challenge. This article provides a summary of recent research trends in such hybrid systems, summarizes the remaining challenges, and points out possible future research directions.
引用
收藏
页码:612 / 626
页数:15
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