INITIO MOLECULAR-DYNAMICS;
TOTAL-ENERGY CALCULATIONS;
OXYGEN EVOLUTION;
SINGLE-ATOM;
TRANSITION;
MXENE;
D O I:
10.1039/d4cp02909g
中图分类号:
O64 [物理化学(理论化学)、化学物理学];
学科分类号:
070304 ;
081704 ;
摘要:
The novel two-dimensional MXene material Ti3C2Tx boasts advantages such as large specific surface area, good electrical conductivity, and high stability, making it suitable for the field of electrocatalysis. However, Ti3C2Tx exhibits unacceptably slow kinetics during the electrocatalytic hydrogen evolution reaction (HER). Electron-metal-support interaction is an effective method for regulating the electronic state of active sites and enhancing HER performance. Therefore, in this study, Fe, Co, and Ni were respectively loaded onto Ti3C2Txvia electron beam deposition to form electron microscopy-supported interface (EMSI) effects, thereby improving the HER activity of Ti3C2Tx. The tests conclude that loading different transition metals (Fe, Co, Ni) onto Ti3C2Tx effectively enhances its HER performance. Experimental and theoretical studies further indicate that the electrocatalytic performance of Ni-loaded Ti3C2Tx is superior to that of Co-loaded and Fe-loaded Ti3C2Tx. This work presents a promising strategy for synthesizing metal-loaded MXene.
机构:
Jilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R ChinaJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
Dai, Mingjun
Zhao, Liupeng
论文数: 0引用数: 0
h-index: 0
机构:
Jilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R ChinaJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
Zhao, Liupeng
Gao, Hongyu
论文数: 0引用数: 0
h-index: 0
机构:
Jilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R ChinaJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
Gao, Hongyu
Sun, Peng
论文数: 0引用数: 0
h-index: 0
机构:
Jilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R ChinaJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
Sun, Peng
Liu, Fengmin
论文数: 0引用数: 0
h-index: 0
机构:
Jilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R ChinaJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
Liu, Fengmin
Zhang, Sean
论文数: 0引用数: 0
h-index: 0
机构:
Jilin Univ, Coll Chem, State Key Lab Supramolecular Struct & Mat, 2699 Qianjin St, Changchun 130012, Peoples R ChinaJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
Zhang, Sean
Shimanoe, Kengo
论文数: 0引用数: 0
h-index: 0
机构:
Kyushu Univ, Fac Engn Sci, Dept Energy & Mat Sci, Kasuga shi, Fukuoka 8168580, JapanJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
Shimanoe, Kengo
Yamazoe, Noboru
论文数: 0引用数: 0
h-index: 0
机构:
Kyushu Univ, Fac Engn Sci, Dept Energy & Mat Sci, Kasuga shi, Fukuoka 8168580, JapanJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
Yamazoe, Noboru
Lu, Geyu
论文数: 0引用数: 0
h-index: 0
机构:
Jilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R ChinaJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Gao, Lei
Bao, Feixiang
论文数: 0引用数: 0
h-index: 0
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Bao, Feixiang
Tan, Xin
论文数: 0引用数: 0
h-index: 0
机构:
Wenzhou Univ, Inst Carbon Neutralizat, Coll Chem & Mat Engn, Wenzhou 325035, Zhejiang, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Tan, Xin
Li, Mengfan
论文数: 0引用数: 0
h-index: 0
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Li, Mengfan
Shen, Zhen
论文数: 0引用数: 0
h-index: 0
机构:
Nanjing Univ, Sch Chem & Chem Engn, MOE, Jiangsu Prov Lab Nanotechnol,Key Lab Mesoscop Chem, Nanjing 210023, Jiangsu, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Shen, Zhen
Chen, Xuli
论文数: 0引用数: 0
h-index: 0
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Chen, Xuli
Tang, Ziyi
论文数: 0引用数: 0
h-index: 0
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Tang, Ziyi
Lai, Wenchuan
论文数: 0引用数: 0
h-index: 0
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Lai, Wenchuan
Lu, Yangfan
论文数: 0引用数: 0
h-index: 0
机构:
Zhejiang Univ, Sch Mat Sci & Engn, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Lu, Yangfan
Huang, Peifeng
论文数: 0引用数: 0
h-index: 0
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Huang, Peifeng
Ma, Chao
论文数: 0引用数: 0
h-index: 0
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Ma, Chao
Smith, Sean C.
论文数: 0引用数: 0
h-index: 0
机构:
Australian Natl Univ, Res Sch Phys, Dept Mat Phys, Integrated Mat Design Lab, Canberra, ACT 2601, AustraliaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Smith, Sean C.
Ye, Zhizhen
论文数: 0引用数: 0
h-index: 0
机构:
Zhejiang Univ, Sch Mat Sci & Engn, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Ye, Zhizhen
Hu, Zheng
论文数: 0引用数: 0
h-index: 0
机构:
Nanjing Univ, Sch Chem & Chem Engn, MOE, Jiangsu Prov Lab Nanotechnol,Key Lab Mesoscop Chem, Nanjing 210023, Jiangsu, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Hu, Zheng
Huang, Hongwen
论文数: 0引用数: 0
h-index: 0
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Hunan Univ, Shenzhen Res Inst, Shenzhen 518055, Guangdong, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
机构:
Jilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R ChinaJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
Dai, Mingjun
Zhao, Liupeng
论文数: 0引用数: 0
h-index: 0
机构:
Jilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R ChinaJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
Zhao, Liupeng
Gao, Hongyu
论文数: 0引用数: 0
h-index: 0
机构:
Jilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R ChinaJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
Gao, Hongyu
Sun, Peng
论文数: 0引用数: 0
h-index: 0
机构:
Jilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R ChinaJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
Sun, Peng
Liu, Fengmin
论文数: 0引用数: 0
h-index: 0
机构:
Jilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R ChinaJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
Liu, Fengmin
Zhang, Sean
论文数: 0引用数: 0
h-index: 0
机构:
Jilin Univ, Coll Chem, State Key Lab Supramolecular Struct & Mat, 2699 Qianjin St, Changchun 130012, Peoples R ChinaJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
Zhang, Sean
Shimanoe, Kengo
论文数: 0引用数: 0
h-index: 0
机构:
Kyushu Univ, Fac Engn Sci, Dept Energy & Mat Sci, Kasuga shi, Fukuoka 8168580, JapanJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
Shimanoe, Kengo
Yamazoe, Noboru
论文数: 0引用数: 0
h-index: 0
机构:
Kyushu Univ, Fac Engn Sci, Dept Energy & Mat Sci, Kasuga shi, Fukuoka 8168580, JapanJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
Yamazoe, Noboru
Lu, Geyu
论文数: 0引用数: 0
h-index: 0
机构:
Jilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R ChinaJilin Univ, College Elect Sci & Engn, 2699 Qianjin St, Changchun 130012, Peoples R China
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Gao, Lei
Bao, Feixiang
论文数: 0引用数: 0
h-index: 0
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Bao, Feixiang
Tan, Xin
论文数: 0引用数: 0
h-index: 0
机构:
Wenzhou Univ, Inst Carbon Neutralizat, Coll Chem & Mat Engn, Wenzhou 325035, Zhejiang, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Tan, Xin
Li, Mengfan
论文数: 0引用数: 0
h-index: 0
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Li, Mengfan
Shen, Zhen
论文数: 0引用数: 0
h-index: 0
机构:
Nanjing Univ, Sch Chem & Chem Engn, MOE, Jiangsu Prov Lab Nanotechnol,Key Lab Mesoscop Chem, Nanjing 210023, Jiangsu, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Shen, Zhen
Chen, Xuli
论文数: 0引用数: 0
h-index: 0
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Chen, Xuli
Tang, Ziyi
论文数: 0引用数: 0
h-index: 0
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Tang, Ziyi
Lai, Wenchuan
论文数: 0引用数: 0
h-index: 0
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Lai, Wenchuan
Lu, Yangfan
论文数: 0引用数: 0
h-index: 0
机构:
Zhejiang Univ, Sch Mat Sci & Engn, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Lu, Yangfan
Huang, Peifeng
论文数: 0引用数: 0
h-index: 0
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Huang, Peifeng
Ma, Chao
论文数: 0引用数: 0
h-index: 0
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Ma, Chao
Smith, Sean C.
论文数: 0引用数: 0
h-index: 0
机构:
Australian Natl Univ, Res Sch Phys, Dept Mat Phys, Integrated Mat Design Lab, Canberra, ACT 2601, AustraliaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Smith, Sean C.
Ye, Zhizhen
论文数: 0引用数: 0
h-index: 0
机构:
Zhejiang Univ, Sch Mat Sci & Engn, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Ye, Zhizhen
Hu, Zheng
论文数: 0引用数: 0
h-index: 0
机构:
Nanjing Univ, Sch Chem & Chem Engn, MOE, Jiangsu Prov Lab Nanotechnol,Key Lab Mesoscop Chem, Nanjing 210023, Jiangsu, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Hu, Zheng
Huang, Hongwen
论文数: 0引用数: 0
h-index: 0
机构:
Hunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China
Hunan Univ, Shenzhen Res Inst, Shenzhen 518055, Guangdong, Peoples R ChinaHunan Univ, Coll Mat Sci & Engn, State Key Lab Adv Design & Mfg Vehicle Body, Changsha 410082, Hunan, Peoples R China