Modulation strategies of metal-organic framework materials and its adsorption performance on typical heavy metal ions

被引:0
|
作者
Chunshu X. [1 ,2 ]
Qingda Y. [2 ,3 ]
Yongxian L. [2 ]
Hualong Z. [2 ,4 ]
机构
[1] Jinjiang Testing Institute of Quality and Metrology, Quanzhou, Fujian
[2] Advanced Polymer Materials Research Center of Sichuan University, Quanzhou, Fujian
[3] Xingye Leather Technology Co., Ltd, Quanzhou, Fujian
[4] National Engineering Laboratory for Clean Technology of Leather Manufacture, Sichuan University, Chengdu, Sichuan
关键词
Adsorption; Heavy metal ions; Metal-organic framework materials; Nanostructure; Stability;
D O I
10.16085/j.issn.1000-6613.2023-0130
中图分类号
学科分类号
摘要
Metal-organic framework materials have the advantages of larger specific surface area, tunable pore and topological structures, and abundant active functional groups compared with traditional adsorbent materials, which can be used as high-performance adsorbents for the removal of heavy metal pollutants from water. In this paper, the structural characteristics of MOFs as adsorbents for water treatment were introduced. The regulatory strategies of MOFs based on metal node doping, side group functionalization and post-synthetic modification, such as porosity, surface activity, framework flexibility, water stability, scalability, biotoxicity and recyclability, were emphatically analyzed. Then, the research progress of MOFs in the removal of heavy metal ions was introduced, mainly on cationic heavy metal ions such as Pb(II) and Hg(II), and anionic oxyanions such as Cr(VI and As(III)/As(V) in water, and the mechanism of the action of MOFs in the removal of heavy metal ions in water was elaborated. Finally, the research directions of improving the water stability and adsorption performance of MOFs, balancing the relationship between the structural characteristics of MOFs, studying the migration and enrichment of MOFs in nature, and the controllable preparation of MOFs with low cost and high benefit were put forward for improving the reference of MOFs in the field of high-performance adsorption. © 2023 Chemical Industry Press. All rights reserved.
引用
收藏
页码:6518 / 6534
页数:16
相关论文
共 98 条
  • [1] HU Shuangyi, ZI Qian, DENG Xiantao, Et al., Application of multielement catalytic oxidation and modified A<sup>2</sup>/O process in the treatment of wastewater from industrial park, China Water & Wastewater, 38, 18, pp. 68-71, (2022)
  • [2] YAO Qingda, WEN Huitao, YANG Changkai, Et al., Structure and performance of multilayer graphene oxide membrane and its application in water treatment: A review, Materials Reports, 34, 15, pp. 15047-15058, (2020)
  • [3] SHENG Mengshuang, YU Mei, SHANG Jing, Et al., High efficient adsorption and photocatalytic removal of hexavalent chromium over three-dimensional graphene oxide aerogel under visible light, Chinese Science Bulletin, 67, pp. 447-458, (2022)
  • [4] ZHANG Lizhu, WANG Huan, LI Qiong, Et al., Research progress on the preparation of lignin-derived adsorption materials and their application in wastewater treatment, Chemical Industry and Engineering Progress, 41, 7, pp. 3731-3744, (2022)
  • [5] YAO Qingda, LIANG Yongxian, WANG Xiaozhuo, Et al., Structure and performance of graphene oxide/chitosan composite and its application in water treatment: A review, Materials Reports, 36, 4, pp. 36-48, (2022)
  • [6] WAN Hongyou, YAN Jingwei, GUO Cong, Et al., A critical review of Cu/Fe-MOF composite materials applied in the water treatment process and its prospect, Technology of Water Treatment, 48, 11, pp. 1-7, (2022)
  • [7] PEI Yuanchao, ZHANG Yaxin, MA Jie, Et al., Carboxyl functional poly (ionic liquid)s confined in metal-organic frameworks with enhanced adsorption of metal ions from water, Separation and Purification Technology, 299, (2022)
  • [8] ZHENG Min, XU Lei, CHEN Chen, Et al., MOFs and GO-based composites as deliberated materials for the adsorption of various water contaminants, Separation and Purification Technology, 294, (2022)
  • [9] SOLTANI Roozbeh, PELALAK Rasool, PISHNAMAZI Mahboubeh, Et al., A water-stable functionalized NiCo-LDH/MOF nanocomposite: Green synthesis, characterization, and its environmental application for heavy metals adsorption, Arabian Journal of Chemistry, 14, 4, (2021)
  • [10] WANG Chongchen, WANG Xun, The application of metal-organic frameworks in the wastewater treatment: A state-of-the-art review, Industrial Water Treatment, 40, 11, pp. 1-9, (2020)