Nonlinear optical characterization of functionalized organometallic complexes using THG and Z-scan techniques

被引：0

作者：

Luc, J. ^{[1
]}

Boudebs, G. ^{[1
]}

Cassagne, C. ^{[1
]}

Fillaut, J.-L. ^{[2
]}

Meghea, A. ^{[3
]}

Rau, I. ^{[3
]}

Migalska-Zalas, A. ^{[4
]}

Bakasse, M. ^{[5
]}

Sahraoui, B. ^{[1
]}

机构：

[1] Laboratoire des Propriétés Optiques des Matériaux et Applications, UMR CNRS 6136, Université d'Angers, 2 boulevard Lavoisier, 49045 Angers Cedex 01, France

[2] Sciences Chimiques de Rennes, UMR CNRS 6226, Campus de Beaulieu, 35042 Rennes Cedex, France

[3] Faculty of Applied Chemistry and Material Science, University Politechnica of Bucharest, Gh Polizu 1, Bucharest, 060032, Romania

[4] Department of Physics, Jan Dlugosz Academy in Czestochowa, al. Armii Krajowej 13/15, Czestochowa PL-42201, Poland

[5] Faculty of Sciences, University Chouaib Doukkali, 24000, El Jadida, Morocco

来源：

Nonlinear Optics Quantum Optics | 2008年 / 38卷 / 02期

关键词：

Chromophores - Yttrium aluminum garnet - Dichloromethane - Organometallics - Refractive index - Neodymium lasers - Nonlinear optics;

D O I：

暂无

中图分类号：

学科分类号：

摘要：

We report the measurements of third-order nonlinear optical (NLO) properties in picosecond regim of functionalized organometallic complexes using third harmonic generation (THG) and Z-scan techniques. We show the results obtained for solutions dissolved in dichloromethane with different concentrations. For each chromophore, we give the values of: the nonlinear absorption coefficient β, the nonlinear refractive index n2, the third-order nonlinear susceptibility χ(3) and the second-order nonlinear hyperpolarisability y of individual molecules. This approach allowed us to determine also the electronic and rotational contributions of χ(3) by using a picosecond laser Nd: YAG at the fundamental wavelength 1064 nm. ©2008 Old City Publishing. Inc.

引用

页码：163 / 173

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