Spatio-temporal Distribution Characteristics of Secondary Aerosol in Beijing-Tianjin-Hebei Urban Agglomeration in Winter

被引:3
|
作者
Yao Q. [1 ,2 ]
Yang X. [1 ,2 ]
Tang Y.-X. [1 ,2 ]
Fan W.-Y. [1 ,2 ]
Cai Z.-Y. [1 ,2 ]
Han S.-Q. [1 ,2 ]
机构
[1] Tianjin Environmental Meteorology Center, Tianjin
[2] CMA-NKU Cooperative Laboratory for Atmospheric Environment-Health Research, Tianjin
来源
Huanjing Kexue/Environmental Science | 2023年 / 44卷 / 05期
关键词
Beijing-Tianjin-Hebei urban agglomeration; ozone(O[!sub]3[!/sub] ); photochemical reaction; secondary aerosol; temporal and spatial distribution;
D O I
10.13227/j.hjkx.202205221
中图分类号
学科分类号
摘要
The secondary component is an important factor causing PM2. 5 pollution in the Beijing-Tianjin-Hebei urban agglomeration in winter. In this study, the CO tracer method was used to estimate the secondary PM2. 5 concentration of the Beijing-Tianjin-Hebei urban agglomeration in the winter of 2017- 2021. The temporal and spatial distribution characteristics were analyzed, and the influencing factors of regional secondary PM2. 5 were discussed. The results showed that the decreasing trend of PM2. 5 concentration in the Beijing-Tianjin-Hebei Region in the winter of 2017-2021 was obvious, and the cities with the largest decline were located in the central and southern part of Hebei Province, mainly contributed by primary PM2. 5 . There was a good correlation between secondary PM2. 5 and PM2. 5 in all cities of the Beijing-Tianjin-Hebei urban agglomeration, and the proportion of secondary PM2. 5 in Beijing and Tianjin was significantly higher than that in other cities. With the aggravation of pollution degree, the mass concentration of primary PM2. 5 and secondary PM2. 5 increased in varying degrees, and the proportion of secondary PM2. 5 increased significantly. Compared with the direct measurement results, the estimated value obtained by this method was lower as a whole. The selection of appropriate primary aerosol reference value was the key to improving this method and estimating the secondary PM2. 5 concentration. © 2023 Science Press. All rights reserved.
引用
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页码:2421 / 2429
页数:8
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  • [1] Li H, Wang S L, Zhang W J, Et al., Characteristics and influencing factors of urban air quality in Beijing-Tianjin-Hebei and its surrounding areas ('2 + 26’ cities), Research of Environmental Sciences, 34, 1, pp. 172-184, (2021)
  • [2] Zhang X Y, Xu X D, Ding Y H, Et al., The impact of meteorological changes from 2013 to 2017 on PM<sub>2. 5</sub> mass reduction in key regions in China, Science China Earth Sciences, 62, 12, pp. 1885-1902, (2019)
  • [3] Cai Z Y, Hao J, Han S Q, Et al., Analysis of change and driving factors of PM<sub>2. 5</sub> mass concentration in Tianjin from 2000 to 2020, Environmental Science, 43, 3, pp. 1129-1139, (2022)
  • [4] Yao Q, Cai Z Y, Liu J L, Et al., Effects of meteorological conditions on PM<sub>2. 5</sub> concentration in Tianjin from 2009 to 2018, Acta Scientiae Circumstantiae, 40, 1, pp. 65-75, (2020)
  • [5] Sun F, Yao H, Liu B X, Et al., Characteristics of PM<sub>2. 5</sub> heavy pollution in Beijing-Tianjin-Hebei and surrounding areas from 2013 to 2019, Environmental Monitoring in China, 37, 4, pp. 46-53, (2021)
  • [6] Dao X, Ji D S, Zhang X, Et al., Characteristics of chemical composition of PM<sub>2. 5</sub> in Beijing-Tianjin-Hebei and its surrounding areas during the heating period, Research of Environmental Sciences, 34, 1, pp. 1-10, (2021)
  • [7] Chang S C, Lee C T., Secondary aerosol formation through photochemical reactions estimated by using air quality monitoring data in Taipei City from 1994 to 2003, Atmospheric Environment, 41, 19, pp. 4002-4017, (2007)
  • [8] Cui H X, Wu Y M, Duan Y S, Et al., Secondary aerosol formation through photochemical reactions estimated by using air quality monitoring data in the downtown of Pudong, Shanghai, Environmental Science, 34, 5, pp. 2003-2009, (2013)
  • [9] Jia M W, Zhao T L, Cheng X H, Et al., Inverse relations of PM<sub>2. 5</sub> and O<sub>3</sub> in air compound pollution between cold and hot seasons over an urban area of east China, Atmosphere, 8, 3, (2017)
  • [10] Li H L, Wang Y J, Huang L, Et al., Analysis of synergistic growth effects between ozone and secondary aerosol in typical cities in China [J], Acta Scientiae Circumstantiae, 40, 12, pp. 4368-4379, (2020)