Surface modification of polyethylene terephthalate films using dielectric barrier discharge driven by repetitive nanosecond pulses

被引:1
作者
Zhang C. [1 ,2 ]
Shao T. [1 ,3 ]
Yu Y. [1 ,2 ]
Long K. [1 ,2 ]
Wang J. [1 ]
Zhang D. [1 ]
Yan P. [1 ]
Zhou Y. [3 ]
机构
[1] Institute of Electrical Engineering, Chinese Academy of Sciences, Beijing 100190
[2] Graduate University of Chinese Academy of Sciences
[3] State Key Laboratory of Control and Simulation of Power System and Generation Equipments, Tsinghua University
来源
Qiangjiguang Yu Lizishu/High Power Laser and Particle Beams | 2010年 / 22卷 / 03期
关键词
Dielectric barrier discharge; Gas discharge; Nanosecond pulse; Repetition rate; Surface modification;
D O I
10.3788/HPLPB20102203.0539
中图分类号
学科分类号
摘要
Surface treatment of polyethylene terephthalate(PET) films for improving the hydrophilicity using dielectric barrier discharge(DBD) excited by unipolar nanosecond pulses is presented. Homogeneous and filamentary discharges are obtained under certain experimental conditions and then used to modify the surface of PET films. The properties of PET films before and after treatment are characterized with water contact angle measurement, atomic force microscope and X-ray photoelectron spectroscope. The experimental results show that static water contact angles decrease evidently after DBD plasma treatment and the observed contact angle changes from 78° for the untreated samples to 25° after treatment. However, the decrease of contact angles is not continuous and it will reach a saturation state after certain treatment time. The improvement of surface hydrophilicity can be attributed to the enhancement of surface roughness and the introduction of oxygen-containing polar functional groups. In contrast with the filamentary DBD treatment, the homogenous DBD is more effective in PET surface treatment.
引用
收藏
页码:539 / 544
页数:5
相关论文
共 19 条
  • [1] Fridman A., Chirokov A., Gutsol A., Non-thermal atmospheric pressure discharges, J Phys D: Appl Phys, 38, (2005)
  • [2] Sung Y.M., Sakoda T., Optimum conditions for ozone formation in a micro dielectric barrier discharge, Surf Coat Technol, 197, pp. 148-153, (2005)
  • [3] Williamson J.M., Trump D.D., Bletzinger P., Et al., Comparison of high-voltage ac and pulsed operation of a surface dielectric barrier discharge, J Phys D: Appl Phys, 39, pp. 4400-4406, (2006)
  • [4] Ono R., Oda T., Ozone production process in pulsed positive dielectric barrier discharge, J Phys D: Appl Phys, 40, pp. 176-182, (2007)
  • [5] Khacef A., Cormier J.M., Pouvesle J.M., NO<sub>x</sub> remediation in oxygen-rich exhaust gas using atmospheric pressure non-thermal plasma generated by a pulsed nanosecond dielectric barrier discharge, J Phys D: Appl Phys, 35, pp. 1491-1498, (2002)
  • [6] Magureanu M., Mandache N.B., Gaigneaux E., Et al., Toluene oxidation in a plasma-catalytic system, J Appl Phys, 99, (2006)
  • [7] Mildren R.P., Carman R.J., Falconer I.S., Visible and VUV emission from a xenon dielectric barrier discharge using pulsed and sinusoidal voltage excitation waveforms, IEEE Trans Plasma Sci, 30, pp. 192-193, (2002)
  • [8] Carman R.J., Mildren R.P., Ward B.K., Et al., High-pressure (>1 bar) dielectric barrier discharge lamps generating short pulses of high-peak power vacuum ultraviolet radiation, J Phys D: Appl Phys, 37, pp. 2399-2407, (2004)
  • [9] Beleznai S., Mihajlik G., Maros I., Et al., Improving the efficiency of a fluorescent Xe dielectric barrier light source using short pulse excitation, J Phys D: Appl Phys, 41, (2008)
  • [10] Ishikawa S., Yukimura K., Matsunaga K., Et al., The surface modification of poly (tetrafluoroethylene) film using dielectric barrier discharge of intermittent pulse voltage, Surf Coat Technol, 130, pp. 52-56, (2000)