Integrated molybdenum single atom array sensors with multichannels for nitrite detection in foods

被引:3
作者
Ding, Mei [1 ]
Tian, Kangling [1 ]
Wang, Jingwen [1 ]
Liu, Yuhang [1 ]
Hu, Guangxuan [1 ]
Zheng, Yan [1 ]
Lei, Shaohui [1 ]
Sun, Jiayue [1 ]
Yang, Hong Bin [1 ]
Hu, Fang Xin [1 ]
机构
[1] Suzhou Univ Sci & Technol, Sch Mat Sci & Engn, Suzhou 215009, JiangSu, Peoples R China
基金
中国国家自然科学基金;
关键词
Nitrite; Array sensor; Molybdenum single atom material; Multiple channels detection; Food detection; ENVIRONMENTAL-SAMPLES; CARBON NANOTUBES; GRAPHENE OXIDE; NITRATE; ELECTROPHORESIS;
D O I
10.1016/j.bios.2024.116345
中图分类号
Q6 [生物物理学];
学科分类号
071011 ;
摘要
Nitrite (NO2- ) is present in a variety of foods, but the excessive intake of NO2- can indirectly lead to carcinogenic, teratogenic, mutagenicity and other risks to the human body. Therefore, the detection of NO(2)(-)is crucial for maintaining human health. In this study, an integrated array sensor for NO2- detection is developed based on molybdenum single atom material (IMSMo-SAC) using high-resolution electrohydrodynamic (EHD) printing technology. The sensor comprises three components: a printed electrode array, multichannels designed on polydimethylsiloxane (PDMS) and an electronic signal process device with bluetooth. By utilizing Mo-SAC to facilitate electron transfer during the redox reaction, rapid and efficient detection of NO2- can be achieved. The sensor has a wide linear range of 0.1 mu M-107.8 mM, a low detection limit of 33 nM and a high sensitivity of 0.637 mA(- 1)mM(- 1) cm(- 2). Furthermore, employing this portable array sensor allows simultaneously measurements of NO(2)( - )concentrations in six different foods samples with acceptable recovery rates. This array sensor holds great potential for detecting of small molecules in various fields.
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页数:8
相关论文
共 43 条
  • [21] Single-atom doping of MoS2 with manganese enables ultrasensitive detection of dopamine: Experimental and computational approach
    Lei, Yu
    Butler, Derrick
    Lucking, Michael C.
    Zhang, Fu
    Xia, Tunan
    Fujisawa, Kazunori
    Granzier-Nakajima, Tomotaroh
    Cruz-Silva, Rodolfo
    Endo, Morinobu
    Terrones, Humberto
    Terrones, Mauricio
    Ebrahimi, Aida
    [J]. SCIENCE ADVANCES, 2020, 6 (32)
  • [22] Bioinspired FeN5 Sites with Enhanced Peroxidase-like Activity Enable Colorimetric Sensing of Uranyl Ions in Seawater
    Li, Ruimin
    Jiao, Lei
    Jia, Xiangkun
    Yan, Lijuan
    Li, Xiaotong
    Yan, Dongbo
    Zhai, Yanling
    Zhu, Chengzhou
    Lu, Xiaoquan
    [J]. ANALYTICAL CHEMISTRY, 2024, 96 (07) : 3124 - 3130
  • [23] Single-Atom Indium Boosts Electrochemical Dopamine Sensing
    Li, Ruimin
    Guo, Weiwei
    Zhu, Zhijun
    Zhai, Yanling
    Wang, Guanwen
    Liu, Zheng
    Jiao, Lei
    Zhu, Chengzhou
    Lu, Xiaoquan
    [J]. ANALYTICAL CHEMISTRY, 2023, 95 (18) : 7195 - 7201
  • [24] Single-Site Sn-O-Cu Pairs with Interfacial Electron Transfer Effect for Enhanced Electrochemical Catalysis and Sensing
    Li, Ruimin
    Guo, Weiwei
    Zhu, Zhijun
    Chen, Yanan
    Jiao, Lei
    Zhu, Chengzhou
    Zhai, Yanling
    Lu, Xiaoquan
    [J]. SMALL, 2023, 19 (27)
  • [25] Lundberg JO, 2008, NAT REV DRUG DISCOV, V7, DOI [10.1038/nrd2466, 10.1038/nrd2466-c2]
  • [26] New development of optical fibre sensor for determination of nitrate and nitrite in water
    Moo, Y. C.
    Matjafri, M. Z.
    Lim, H. S.
    Tan, C. H.
    [J]. OPTIK, 2016, 127 (03): : 1312 - 1319
  • [27] Nitrogen reduction by the Fe sites of synthetic [Mo3S4Fe] cubes
    Ohki, Yasuhiro
    Munakata, Kenichiro
    Matsuoka, Yuto
    Hara, Ryota
    Kachi, Mami
    Uchida, Keisuke
    Tada, Mizuki
    Cramer, Roger E.
    Sameera, W. M. C.
    Takayama, Tsutomu
    Sakai, Yoichi
    Kuriyama, Shogo
    Nishibayashi, Yoshiaki
    Tanifuji, Kazuki
    [J]. NATURE, 2022, 607 (7917) : 86 - +
  • [28] Measuring Electrochemical Surface Area of Nanomaterials versus the Randles-Sevcik Equation
    Paixao, Thiago R. L. C.
    [J]. CHEMELECTROCHEM, 2020, 7 (16): : 3414 - 3415
  • [29] Oxidation of nitrites on solid electrodes - I. Determination of the reaction mechanism on the pure electrode surface
    Piela, B
    Wrona, PK
    [J]. JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2002, 149 (02) : E55 - E63
  • [30] Single-atom catalysts reveal the dinuclear characteristic of active sites in NO selective reduction with NH3
    Qu, Weiye
    Liu, Xiaona
    Chen, Junxiao
    Dong, Yangyang
    Tang, Xingfu
    Chen, Yaxin
    [J]. NATURE COMMUNICATIONS, 2020, 11 (01)