Effects of Oxygen Volume Fraction on Morphology and Particle Size Evolution of Soot in Laminar Coflow Ethylene Diffusion Flames

被引:0
|
作者
Han W.-W. [1 ]
Cao W.-J. [1 ]
Chu H.-Q. [1 ]
Gu M.-Y. [1 ]
机构
[1] School of Energy and Environment, Anhui University of Technology, Ma'anshan
来源
Chu, Hua-Qiang (hqchust@163.com) | 2018年 / Journal of Propulsion Technology卷 / 39期
关键词
Deposit morphology; Laminar diffusion flame; Oxygen volume fraction; Soot; Temperature;
D O I
10.13675/j.cnki.tjjs.2018.12.018
中图分类号
学科分类号
摘要
In order to study the effects of oxygen volume fraction on the formation and evolution of soot particles in laminar coflow diffusion flames of ethylene, SiC fiber deposition and thermophoresis probe sampling methods were used to investigate the soot characteristics at different radial and axial positions in laminar diffusion flame. The results demonstrate that the temperature increases with increasing the oxygen volume fraction at the same location. When the oxygen volume fraction is less than 31% and the flame height is lower than 30mm, the morphology of the soot deposits on the SiC fiber evolves gradually from smooth droplet-like at the centerline to uneven clusters at larger radical locations. With increasing temperature and enhanced role of oxidation, the morphology of soot deposits on the SiC fiber is gradually oxidized into loose cluster-like, flocculent, and final transition to dense clusters and fiber mesh. Under the constant oxygen volume fraction, the average particle size of soot particles increases first and then decreases with the increase of flame height. The diameter of primary particles reached the maximum at 21% oxygen volume fraction and flame height 30mm, which was 41.8nm. At the base of the flame, the average soot particle size increased with the increase of oxygen concentration, the opposite trend was observed at higher flame heights. © 2018, Editorial Department of Journal of Propulsion Technology. All right reserved.
引用
收藏
页码:2788 / 2797
页数:9
相关论文
共 42 条
  • [1] Lee K.O., Megaridis M.C., Zelepouga S., Et al., Soot Formation Effects of Oxygen Concentration in the Oxidizer Stream of Laminar Coannular Nonpremixed Methane/Air Flames, Combustion and Flame, 121, 1-2, pp. 323-333, (2000)
  • [2] Liu Y.-Y., Li N.-N., Huang W.-Q., Review on Soot Radiation Property Estimation of Combustion Process, Journal of Propulsion Technology, 37, 3, pp. 479-487, (2016)
  • [3] Ramanathan V., Carmichael G., Global and Regional Climate Changes Due to Black Carbon, Nature Geoscience, 36, 1, pp. 335-358, (2008)
  • [4] Jacobson M.Z., Strong Radiative Heating Due to the Mixing State of Black Carbon in Atmospheric Aerosols, Nature, 409, 6, pp. 695-697, (2001)
  • [5] Zhang X.-T., Song W.-L., Guo L.-G., Et al., Preparation of Carbon-Coated Al Nanopowders by Laser-Induction Complex Heating Method, Journal of Propulsion Technology, 28, 3, pp. 333-336, (2007)
  • [6] Glassman I., Soot Formation in Combustion Processes, Symposium on Combustion, 22, 1, pp. 295-311, (1989)
  • [7] Santoro R.J., Yeh T.T., Horvath J.J., Et al., The Transport and Growth of Soot Particles in Laminar Diffusion Flames, Combustion Science and Technology, 53, 2-3, pp. 89-115, (1987)
  • [8] Wang H., Frenklach M., A Detailed Kinetic Modeling Study of Aromatics Formation in Laminar Premixed Acetylene and Ethylene Flames, Combustion and Flame, 110, 1-2, pp. 173-221, (1997)
  • [9] Richter H., Howard J.B., Formation of Polycyclic Aromatic Hydrocarbons and Their Growth to Soot-a Review of Chemical Reaction Pathways, Journal of Applied Polymer Science, 26, 4, pp. 565-608, (2000)
  • [10] Howard J.B., Chowdhury K.D., Vander Sande J.B., Carbon Shells in Flames, Nature, 370, 6491, (1994)