A Review of Metal-Organic Frameworks Derived Hollow-Structured Photocatalysts: Synthesis and Applications

被引：0
作者：
Tang, Chenxi [1 ]
Rao, Heng [1 ]
Li, Shuming [1 ]
She, Ping [1 ,2 ]
Qin, Jun-sheng [1 ]
机构：
[1] Jilin Univ, Coll Chem, Int Ctr Future Sci, State Key Lab Inorgan Synth & Preparat Chem, 2699 Qianjin St, Changchun 130012, Peoples R China
[2] Jilin Univ, Coll Chem, Key Lab Supramol Struct & Mat, Changchun 130012, Peoples R China
来源：
SMALL | 2024年 / 20卷 / 48期
基金：
中国国家自然科学基金;
关键词：
hollow-structured materials; MOFs; photocatalysis; semiconductor; GRAPHITIC CARBON NITRIDE; ZEOLITIC IMIDAZOLATE FRAMEWORKS; S-SCHEME HETEROJUNCTION; VISIBLE-LIGHT; CORE-SHELL; CHARGE SEPARATION; NITROGEN-FIXATION; OXYGEN REDUCTION; EFFICIENT; WATER;
D O I：
10.1002/smll.202405533
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
Photocatalysis is a most important approach to addressing global energy shortages and environmental issues due to its environmentally friendly and sustainable properties. The key to realizing efficient photocatalysis relies on developing appropriate catalysts with high efficiency and chemical stability. Among various photocatalysts, Metal-organic frameworks (MOFs)-derived hollow-structured materials have drawn increased attention in photocatalysis based on advantages like more active sites, strong light absorption, efficient transfer of pho-induced charges, excellent stability, high electrical conductivity, and better biocompatibility. Specifically, MOFs-derived hollow-structured materials are widely utilized in photocatalytic CO2 reduction (CO2RR), hydrogen evolution (HER), nitrogen fixation (NRR), degradation, and other reactions. This review starts with the development story of MOFs, the commonly adopted synthesis strategies of MOFs-derived hollow materials, and the latest research progress in various photocatalytic applications are also introduced in detail. Ultimately, the challenges of MOFs-derived hollow-structured materials in practical photocatalytic applications are also prospected. This review holds great potential for developing more applicable and efficient MOFs-derived hollow-structured photocatalysts. This review starts with the development story of MOFs, the commonly adopted synthesis strategies of MOFs-derived hollow materials, and the latest research progress in various photocatalytic applications are also introduced in detail. Finally, the challenges of MOFs-derived hollow-structured materials in practical photocatalytic applications are also prospected. This review holds great potential for developing more applicable and efficient MOFs-derived hollow-structured photocatalysts. image
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页数：24
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