Porphyrin-linked graphdiyne as a substrate for constructing single-atom catalysts with transition metals towards oxygen reduction reactions and oxygen evolution reactions

被引：0
作者：
Ping, Jiejie [1 ]
Wu, Mei [2 ]
Liu, Manyu [1 ]
Jiang, Yan [1 ]
Shang, Wenhui [1 ]
Jiao, Menggai [3 ]
Ruan, Jiahao [2 ]
Wang, Nan [1 ]
Jia, Zhiyu [1 ]
机构：
[1] Beijing Inst Technol, Sch Chem & Chem Engn, Key Lab Cluster Sci,Minist Educ, Key Lab Photoelect Electrophoton Convers Mat, Beijing 100081, Peoples R China
[2] China Univ Petr Beijing Karamay, Sch Engn, Karamay 834000, Xinjiang, Peoples R China
[3] Zhengzhou Univ, Interdisciplinary Res Ctr Sustainable Energy Sci &, Sch Chem Engn, Zhengzhou 45001, Peoples R China
来源：
MATERIALS CHEMISTRY FRONTIERS | 2024年 / 8卷 / 22期
基金：
中国国家自然科学基金;
关键词：
FUEL-CELLS; POLYMER; METALLOPORPHYRINS; ELECTROCATALYST; PERFORMANCE; DESIGN; IRON;
D O I：
10.1039/d4qm00555d
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
Porphyrin-linked graphdiyne (PGDY) is a carbon-based material that provides a platform for anchoring single-atom catalysts (SACs) with transition metals (TMs). These SACs have the potential to boost the catalytic activity of the PGDY substrate. The synthesized TM@PGDY composites showed remarkable catalytic activity towards oxygen reduction reactions and oxygen evolution reactions. Porphyrin-linked graphdiyne anchored with transition metals exhibits outstanding electrochemical performance, attributed to the modifications in the coordination environment.
引用
收藏
页码：3741 / 3746
页数：6
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