Preparation and characterization of biochar from four different solid wastes and its ampicillin adsorption performance

被引:0
作者
Yu, Junxin [1 ]
Gu, Tianyu [1 ]
Wang, Ruiying [1 ]
Li, Bing [1 ]
Dong, Zhiying [1 ]
Zhu, Xiaohui [1 ]
Li, Zhexuan [1 ]
Hu, Tiantian [1 ]
Huang, Ying [1 ]
机构
[1] Ningbo Univ, Sch Civil & Environm Engn & Geog Sci, Ningbo 315000, Zhejiang, Peoples R China
关键词
Adsorption; Ampicillin; Biochar; Solid waste; Mechanism; ACTIVATED CARBON; REMOVAL; WATER; TETRACYCLINE; COMPOSITE; MECHANISM; BEHAVIOR; SORPTION; RELEASE;
D O I
10.1007/s10653-024-02221-x
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The integration of biochar (BC) production from organic waste with ampicillin (AMP), an emerging pollutant, adsorption is a novel and promising treatment approach. In this study, peanut shells, coffee grounds, digestates, and oyster shells were used for BC production. Among these, the use of anaerobic digestate from food waste fermentation to produce extracts for antibiotic adsorption is relatively unexplored. The pyrolysis temperature was determined using thermogravimetric analysis (TGA) and the materials were characterized with BET, SEM, FTIR, and XRD. The TGA results indicate that PSB, CRB, and DSB underwent pyrolysis involving cellulose, hemicellulose, and lignin, whereas OSB underwent crystal formation. Characterization revealed that DSB has more functional groups, a superior mesoporous structure, appropriate O/C ratio, and trace amounts of calcite crystals, which are favorable for AMP adsorption. Adsorption experiments demonstrate that all four materials adhere to the Freundlich and Langmuir isotherm and Elovich kinetic models, indicating predominant physical adsorption, with some chemical adsorption also present. Thermodynamic studies demonstrate that BC is spontaneous during adsorption and is a heat-absorbing reaction. DSB exhibits the strongest AMP adsorption. A 53.81 mg g-1 adsorbance was obtained at a dosage of 150 mg, pH = 2, and 60 degrees C. This study introduces innovative approaches for managing waste types and provides data to support the selection of suitable solid wastes for the preparation of BC with excellent adsorption properties. Furthermore, it lays the groundwork for future studies aimed at enhancing the AMP treatment efficacy.Graphical Abstract Preparation and characterization of biochar and adsorption mechanism of ampicillin in water.
引用
收藏
页数:21
相关论文
共 76 条
  • [11] Preparation and characterization of activated carbon from cotton stalk by microwave assisted chemical activation-Application in methylene blue adsorption from aqueous solution
    Deng, Hui
    Yang, Le
    Tao, Guanghui
    Dai, Jiulei
    [J]. JOURNAL OF HAZARDOUS MATERIALS, 2009, 166 (2-3) : 1514 - 1521
  • [12] Review: Micro-organic contaminants in groundwater in China
    Dong, Weihong
    Xie, Wei
    Su, Xiaosi
    Wen, Chuanlei
    Cao, Zhipeng
    Wan, Yuyu
    [J]. HYDROGEOLOGY JOURNAL, 2018, 26 (05) : 1351 - 1369
  • [13] A review of antibiotics and antibiotic resistance genes (ARGs) adsorption by biochar and modified biochar in water
    Du, Linqing
    Ahmad, Shakeel
    Liu, Linan
    Wang, Lan
    Tang, Jingchun
    [J]. SCIENCE OF THE TOTAL ENVIRONMENT, 2023, 858
  • [14] Biochar application to low fertility soils: A review of current status, and future prospects
    El-Naggar, Ali
    Lee, Sang Soo
    Rinklebe, Joerg
    Farooq, Muhammad
    Song, Hocheol
    Sarmah, Ajit K.
    Zimmerman, Andrew R.
    Ahmad, Mahtab
    Shaheen, Sabry M.
    Ok, Yong Sik
    [J]. GEODERMA, 2019, 337 : 536 - 554
  • [15] European Medicines Agency, 2021, Sales of Veterinary Antimicrobial Agents in 31 European Countries in 2019 and 2020 (EMA/294674/2019)
  • [16] Mechanism and behavior of caffeine sorption: affecting factors
    Fakioglu, Merve
    Kalpakli, Yasemen
    [J]. RSC ADVANCES, 2022, 12 (41) : 26504 - 26513
  • [17] Freundlich H., 1907, J. Phys. Chem., V57, P385, DOI DOI 10.1515/ZPCH-1907-5723
  • [18] Obtention of biochar-Fe/Ce using Punica granatum with high adsorption of ampicillin capacity
    Gomez-Vilchis, J. C.
    Garcia-Rosales, G.
    Longoria-Gandara, L. C.
    Perez-Gomez, E. O.
    Castilleros, D. T.
    [J]. HELIYON, 2022, 8 (01)
  • [19] Natural adsorption of methylene blue by waste fallen leaves of Magnoliaceae and its repeated thermal regeneration for reuse
    Guo, Dabin
    Li, Yuexin
    Cui, Baihui
    Hu, Mian
    Luo, Shiyi
    Ji, Bin
    Liu, Yu
    [J]. JOURNAL OF CLEANER PRODUCTION, 2020, 267
  • [20] Interactive effects of biochar and mussel shell activated concoctions on immobilization of nickel and their amelioration on the growth of rapeseed in contaminated aged soil
    Hannan, Fakhir
    Islam, Faisal
    Huang, Qian
    Farooq, Muhammad A.
    Ayyaz, Ahsan
    Fang, Rouyi
    Ali, Basharat
    Xie, Xiaohong
    Zhou, Weijun
    [J]. CHEMOSPHERE, 2021, 282