Solid-State Electrolytes: Probing Interface Regulation from Multiple Perspectives

被引:1
作者
Zhu, Yuchuan [1 ]
Wang, Cong [1 ]
Guo, Daying [1 ]
Chen, Xian [1 ]
Wang, Shun [1 ]
机构
[1] Wenzhou Univ, Coll Chem & Mat Engn, Key Lab Carbon Mat Zhejiang Prov, Wenzhou 325035, Peoples R China
关键词
Solid-state electrolytes; Interfacial engineering; Interlayers; Regulate strategies; Lithium batteries; COMPOSITE POLYMER ELECTROLYTE; LITHIUM METAL ANODE; HIGH-ENERGY; BATTERIES; CONDUCTIVITY; CHALLENGES; NANOSPHERES; STABILITY; MECHANISM; CLUSTERS;
D O I
10.1021/acsami.4c07428
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Solid-state electrolytes (SSEs), as the heart of all-solid-state batteries (ASSBs), are recognized as the next-generation energy storage solution, offering high safety, extended cycle life, and superior energy density. SSEs play a pivotal role in ion transport and electron separation. Nonetheless, interface compatibility and stability issues pose significant obstacles to further enhancing ASSB performance. Extensive research has demonstrated that interface control methods can effectively elevate ASSB performance. This review delves into the advancements and recent progress of SSEs in interfacial engineering over the past years. We discuss the detailed effects of various regulation strategies and directions on performance, encompassing enhancing Li+ mobility, reducing energy barriers, immobilizing anions, introducing interlayers, and constructing unique structures. This review offers fresh perspectives on the development of high-performance lithium-metal ASSBs.
引用
收藏
页码:43114 / 43133
页数:20
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