Stable superhydrophobic interfacial solar evaporator based on CuS@CDs hybrid photothermal composites towards ultrahigh-efficiency seawater evaporation

被引:4
|
作者
Wu, Wanze [1 ]
Han, Xinting [1 ]
Gong, Xiao [1 ,2 ]
机构
[1] Wuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R China
[2] Qingdao Univ, State Key Lab Biofibers & Ecotext, Qingdao 430070, Peoples R China
关键词
Superhydrophobic; Solar evaporator; Photothermal; Seawater desalination; STEAM-GENERATION; HIGHLY EFFICIENT; DESALINATION; SPONGE; FOAM;
D O I
10.1016/j.apenergy.2024.124099
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
Superhydrophobic evaporator driven by solar energy is very promising in seawater desalination. However, low evaporation rate and photothermal conversion efficiency have greatly limited its practical applications. Here, we report a stable superhydrophobic solar evaporator with excellent photothermal performance for efficient saline evaporation. Specifically, CuS@carbon dots (CDs) composites are synthesized by a facile one-step hydrothermal approach. Then the composites are combined with fluorocarbon resin (FEVE) and sprayed on melamine sponge surface to create hierarchical structure to construct a superhydrophobic solar evaporator. Its excellent photothermal properties result from the synergistic effect of CuS and CDs in the composites. The temperature of the evaporator upper surface can rise to 125 degrees C within 3 min, and the evaporator presents high solar-vapor conversion efficiency (77.3%) and water evaporation rate (1.76 kg center dot m- 2 center dot h- 1) under 1.5 Sun. Excitingly, for saline, the evaporation rate remains little changed (1.71 kg center dot m- 2 center dot h- 1). Even after 10 test cycles (300 min), the evaporation rate of saline water is still able to reach 1.40 kg center dot m- 2 center dot h- 1. Furthermore, the evaporator keeps hydrophobic property after being continuously immersed in high-concentration saline for 40 days, exhibiting excellent salt resistance. The prepared superhydrophobic evaporator with excellent photothermal performance has great potential in the fields of seawater desalination and sewage treatment.
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页数:13
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