Decreased nitrogen deposition in Beijing over the recent decade and its implications

被引：0

作者：

Si, Ruotong ^{[1
]}

Yu, Ziyin ^{[1
]}

Ma, Xin ^{[1
]}

Wen, Zhang ^{[1
]}

Luo, Ting ^{[1
]}

Xu, Wen ^{[1
]}

Liu, Lei ^{[1
]}

Tang, Aohan ^{[1
]}

Wang, Kai ^{[1
]}

Zhang, Lin ^{[2
]}

Schweiger, Andreas ^{[3
]}

Goulding, Keith ^{[4
]}

Liu, Xuejun ^{[1
]}

机构：

[1] China Agr Univ, Natl Acad Green Agr Dev, Coll Resources & Environm Sci, State Key Lab Nutrient Use & Management, Beijing 100193, Peoples R China

[2] Peking Univ, Sch Phys, Dept Atmospher & Ocean Sci, Beijing 100871, Peoples R China

[3] Univ Hohenheim, Inst Landscape & Plant Ecol, Dept Plant Ecol, D-70599 Stuttgart, Germany

[4] Rothamsted Res, Sustainable Soils & Crops, Harpenden AL5 2JQ, England

来源：

SCIENCE OF THE TOTAL ENVIRONMENT | 2024年 / 948卷

基金：

中国国家自然科学基金;

关键词：

Nitrogen deposition; Policy regulation; Air quality; Emissions; Beijing; DRY DEPOSITION; ATMOSPHERIC NITROGEN; SOURCE APPORTIONMENT; UNITED-STATES; AIR-QUALITY; CHINA; PRECIPITATION; AMMONIA; SULFUR; WET;

D O I：

10.1016/j.scitotenv.2024.174808

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

Atmospheric reactive nitrogen (Nr) deposition has been modified significantly by human activities such as agriculture and fossil fuel combustion. Understanding the changes in Nr deposition is essential for maintaining the functionality and sustainability of ecosystems. Taking Beijing as a case study, we report long-term measurements of wet Nr deposition from 1999 to 2022 and dry Nr deposition from 2010 to 2022 and their relationship with China's air pollution control. Total Nr deposition to Beijing decreased by 34 % during 2010-2022, mainly caused by a decrease in dry N deposition by 54.27%, from 47.86 kg N ha(-1) yr(-1) in 2010-2014 to 21.89 kg N ha(-1) yr(-1) in 2018-2022; reduced and oxidized N in dry deposition decreased by 29.93 % and 72.05 %, respectively. This was a result of the "Action Plan for Prevention and Control of Air Pollution (APCP)" and the implementation of the "Zero Growth in Fertilizer Use by 2020" in 2015. Our ground-based measurements provide evidence to support recent achievements in air pollution control and a reference and guidance for other regions of China and other countries for abating Nr pollution.

引用

页数：9

共 53 条

[1] Global Estimates of Inorganic Nitrogen Deposition Across Four Decades [J].

Ackerman, Daniel ;

Millet, Dylan B. ;

Chen, Xin .

GLOBAL BIOGEOCHEMICAL CYCLES, 2019, 33 (01) :100-107

[2] Long-term regional trends of nitrogen and sulfur deposition in the United States from 2002 to 2017 [J].

Benish, Sarah E. ;

Bash, Jesse O. ;

Foley, Kristen M. ;

Appel, K. Wyat ;

Hogrefe, Christian ;

Gilliam, Robert ;

Pouliot, George .

ATMOSPHERIC CHEMISTRY AND PHYSICS, 2022, 22 (19) :12749-12767

[3] Characteristics and sources of submicron aerosols above the urban canopy (260 m) in Beijing, China, during the 2014 APEC summit [J].

Chen, C. ;

Sun, Y. L. ;

Xu, W. Q. ;

Du, W. ;

Zhou, L. B. ;

Han, T. T. ;

Wang, Q. Q. ;

Fu, P. Q. ;

Wang, Z. F. ;

Gao, Z. Q. ;

Zhang, Q. ;

Worsnop, D. R. .

ATMOSPHERIC CHEMISTRY AND PHYSICS, 2015, 15 (22) :12879-12895

[4] Mapping global soil acidification under N deposition [J].

Chen, Chen ;

Xiao, Wenya ;

Chen, Han Y. H. .

GLOBAL CHANGE BIOLOGY, 2023, 29 (16) :4652-4661

[5] Mapping N deposition impacts on soil microbial biomass across global terrestrial ecosystems [J].

Chen, Chen ;

Chen, Xinli ;

Chen, Han Y. H. .

GEODERMA, 2023, 433

[6] Loss of plant species after chronic low-level nitrogen deposition to prairie grasslands [J].

Clark, Christopher M. ;

Tilman, David .

NATURE, 2008, 451 (7179) :712-715

[7] Nitrogen and sulfur deposition on regional and global scales:: A multimodel evaluation [J].

Dentener, F. ;

Drevet, J. ;

Lamarque, J. F. ;

Bey, I. ;

Eickhout, B. ;

Fiore, A. M. ;

Hauglustaine, D. ;

Horowitz, L. W. ;

Krol, M. ;

Kulshrestha, U. C. ;

Lawrence, M. ;

Galy-Lacaux, C. ;

Rast, S. ;

Shindell, D. ;

Stevenson, D. ;

Van Noije, T. ;

Atherton, C. ;

Bell, N. ;

Bergman, D. ;

Butler, T. ;

Cofala, J. ;

Collins, B. ;

Doherty, R. ;

Ellingsen, K. ;

Galloway, J. ;

Gauss, M. ;

Montanaro, V. ;

Mueller, J. F. ;

Pitari, G. ;

Rodriguez, J. ;

Sanderson, M. ;

Solmon, F. ;

Strahan, S. ;

Schultz, M. ;

Sudo, K. ;

Szopa, S. ;

Wild, O. .

GLOBAL BIOGEOCHEMICAL CYCLES, 2006, 20 (04)

[8] Ammonia Emission Measurements for Light-Duty Gasoline Vehicles in China and Implications for Emission Modeling [J].

Huang, Cheng ;

Hu, Qingyao ;

Lou, Shengrong ;

Tian, Junjie ;

Wang, Ruinin ;

Xu, Chong ;

An, Jingyu ;

Ren, Hongjuan ;

Ma, Dong ;

Quan, Yifeng ;

Zhang, Yaojiao ;

Li, Li .

ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2018, 52 (19) :11223-11231

[9] Wet deposition of inorganic ions in 320 cities across China: spatio-temporal variation, source apportionment, and dominant factors [J].

Li, Rui ;

Cui, Lulu ;

Zhao, Yilong ;

Zhang, Ziyu ;

Sun, Tianming ;

Li, Junlin ;

Zhou, Wenhui ;

Meng, Ya ;

Huang, Kan ;

Fu, Hongbo .

ATMOSPHERIC CHEMISTRY AND PHYSICS, 2019, 19 (17) :11043-11070

[10] Exploring global changes in agricultural ammonia emissions and their contribution to nitrogen deposition since 1980 [J].

Liu, Lei ;

Xu, Wen ;

Lu, Xiankai ;

Zhong, Buqing ;

Guo, Yixin ;

Lu, Xiao ;

Zhao, Yuanhong ;

He, Wei ;

Wang, Songhan ;

Zhang, Xiuying ;

Liu, Xuejun ;

Vitousek, Peter .

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2022, 119 (14)

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