Enhanced corrosion resistance of AZ31 Mg alloy by one-step formation of PEO/Mg-Al LDH composite coating

被引:61
作者
Zhang, Xinxin [1 ,2 ]
Zhang, Yupeng [1 ,2 ]
Lv, You [1 ,2 ]
Dong, Zehua [1 ]
Hashimoto, Teruo [3 ]
Zhou, Xiaorong [3 ]
机构
[1] Huazhong Univ Sci & Technol, Sch Chem & Chem Engn, Serv Failure, Key Lab Mat Chem Energy Convers & Storage,,Minist, Wuhan 430074, Peoples R China
[2] Huazhong Univ Sci & Technol, Hubei Engn Res Ctr Biomat & Med Protect Mat, Wuhan 430074, Peoples R China
[3] Univ Manchester, Corros & Protect Ctr, Dept Mat, Manchester M13 9PL, England
基金
中国国家自然科学基金;
关键词
AZ31 Mg alloy; Plasma electrolytic oxidation; Layered double hydroxide; Corrosion resistance; PLASMA ELECTROLYTIC OXIDATION; MICRO-ARC OXIDATION; BIODEGRADABLE MAGNESIUM ALLOYS; ANODIC-OXIDATION; PURE MAGNESIUM; IRON CONTENT; BEHAVIOR; SURFACE; ENRICHMENT; COPPER;
D O I
10.1016/j.corcom.2022.05.001
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
In the present work, a novel one-step plasma electrolytic oxidation (PEO) method is developed for the formation of PEO/Mg-Al layered double hydroxide (LDH) composite coating on AZ31 Mg alloy. Through the control of electrolyte concentration, a Mg-Al LDH layer was formed on the surface of the resultant PEO coating. The corrosion properties of the composite coating were evaluated by electrochemical analysis, hydrogen evolution measurement and salt spraying testing, which exhibited improved corrosion resistance due to the presence of the Mg-Al LDH layer. This work provides a new strategy to take advantage of alloying elements in Mg alloys in PEO treatment to enhance corrosion resistance. (c) 2022 The Author(s). Published by Elsevier B.V. on behalf of Institute of Metal Research, Chinese Academy of Sciences. This is an open access article under the CC BY license ( http://creativecommons.org/licenses/by/4.0/ )
引用
收藏
页码:67 / 83
页数:17
相关论文
共 82 条
[1]   Biodegradable magnesium alloys for orthopaedic applications: A review on corrosion, biocompatibility and surface modifications [J].
Agarwal, Sankalp ;
Curtin, James ;
Duffy, Brendan ;
Jaiswal, Swarna .
MATERIALS SCIENCE & ENGINEERING C-MATERIALS FOR BIOLOGICAL APPLICATIONS, 2016, 68 :948-963
[2]   Surface modification and cytotoxicity of Mg-based bio-alloys: An overview of recent advances [J].
Ali, Murad ;
Elsherif, Mohamed ;
Salih, Ahmed E. ;
Ul-Hamid, Anwar ;
Hussein, M. A. ;
Park, Seongjun ;
Yetisen, Ali K. ;
Butt, Haider .
JOURNAL OF ALLOYS AND COMPOUNDS, 2020, 825
[3]   Review of Mg alloy corrosion rates [J].
Atrens, Andrej ;
Shi, Zhiming ;
Mehreen, Syeda U. ;
Johnston, Sean ;
Song, Guang-Ling ;
Chen, Xianhua ;
Pan, Fusheng .
JOURNAL OF MAGNESIUM AND ALLOYS, 2020, 8 (04) :989-998
[4]   Increasing the application fields of magnesium by ultraceramic®: Corrosion and wear protection by plasma electrolytical oxidation (PEO) of Mg alloys [J].
Buling, Anna ;
Zerrer, Joerg .
SURFACE & COATINGS TECHNOLOGY, 2019, 369 :142-155
[5]   The effect of substrate composition on the electrochemical and mechanical properties of PEO coatings on Mg alloys [J].
Cakmak, Emrah ;
Tekin, Kadir C. ;
Malayoglu, Ugur ;
Shrestha, Suman .
SURFACE & COATINGS TECHNOLOGY, 2010, 204 (08) :1305-1313
[6]   Corrosion resistance of thermally sprayed Al and Al/SiC coatings on Mg [J].
Campo, M. ;
Carboneras, M. ;
Lopez, M. D. ;
Torres, B. ;
Rodrigo, P. ;
Otero, E. ;
Rams, J. .
SURFACE & COATINGS TECHNOLOGY, 2009, 203 (20-21) :3224-3230
[7]   Effect of alloy cations on corrosion resistance of LDH/MAO coating on magnesium alloy [J].
Chen, Junfeng ;
Lin, Wenxin ;
Liang, Shiyan ;
Zou, Linchi ;
Wang, Chen ;
Wang, Binshu ;
Yan, Mufu ;
Cui, Xiping .
APPLIED SURFACE SCIENCE, 2019, 463 :535-544
[8]   Influence of second phase on corrosion performance and formation mechanism of PEO coating on AZ91 Mg alloy [J].
Chen, Yan ;
Yang, Yange ;
Zhang, Wei ;
Zhang, Tao ;
Wang, Fuhui .
JOURNAL OF ALLOYS AND COMPOUNDS, 2017, 718 :92-103
[9]   3-D distribution characteristics of the micro-defects in the PEO coating on ZM6 mg-alloy during corrosion [J].
Chen, Zhenning ;
Ji, Haotian ;
Geng, Xiaoqian ;
Chen, Xiaochun ;
Yong, Xingyue ;
Zhang, Suode .
CORROSION SCIENCE, 2020, 174
[10]   Antibacterial activities and corrosion behavior of novel PEO/nanostructured ZrO2 coating on Mg alloy [J].
Daroonparvar, Mohammadreza ;
Mat Yajid, Muhamad Azizi ;
Kumar Gupta, Rajeev ;
Mohd Yusof, Noordin ;
Bakhsheshi-Rad, Hamid Reza ;
Ghandvar, Hamidreza ;
Ghasemi, Ehsan .
TRANSACTIONS OF NONFERROUS METALS SOCIETY OF CHINA, 2018, 28 (08) :1571-1581