Sensitive Breath Acetone Detection Based on α-Fe2O3 Nanoparticles Modified WO3 Nanoplate Heterojunctions

被引:36
作者
Yu, Chenyang [1 ]
Liu, Jianhong [1 ]
Zhao, Hongchao [1 ]
Wang, Mengqing [1 ]
Li, Jing [1 ]
She, Xiaopeng [1 ]
Chen, Yi [1 ]
Wang, Yangjie [1 ]
Liu, Bochao [1 ]
Zou, Cheng [2 ]
He, Yong [1 ]
Zhou, Yong [1 ]
机构
[1] Chongqing Univ, Coll Optoelect Engn, Key Lab Optoelect Technol & Syst, Minist Educ, Chongqing 400044, Peoples R China
[2] Chongqing Univ, Innovat Drug Res Ctr, Sch Pharmaceut Sci, Chongqing Key Lab Nat Prod Synth & Drug Res, Chongqing 401331, Peoples R China
关键词
Iron; Sensors; Temperature sensors; Metals; Adsorption; Nanoparticles; Heterojunctions; Acetone detection; conductometric gas sensors; heterojunctions; tungsten trioxide (WO3) nanoplates; alpha-Fe2O3; SENSING PERFORMANCE; ZINC FERRITE; SENSORS; NANOCOMPOSITES; DESIGN;
D O I
10.1109/TIM.2024.3440407
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
Acetone plays a critical role in environmental protection and human healthcare, thus necessitating sensitive and selective detection. In this regard, a resistive microelectromechanical system (MEMS) acetone sensor featuring a sensing layer of alpha -Fe(2)O(3)nanoparticles modified tungsten trioxide (WO3) nanoplates is utilized in this work. After optimizing the composition proportion and operating temperature, the Fe/W:0.2 sensor delivered a wide detection range (0.05-80 ppm), and an approximately sevenfold higher response of 40.6 toward 10 ppm acetone at 217 degrees C than pure WO3 analog. In addition, a limit of detection (LoD) of 50 ppb was achieved, which ranks among the lowest cases thus far. Together with excellent repeatability, selectivity, and long-term stability, the sensor also showed a humidity-enhanced response. This work offers an alternative strategy to realize trace acetone detection within high-humidity conditions and showcases a huge application potential in exhaled breath-involving diabetes monitoring in the future.
引用
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页数:8
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