Colossal Orbital Current Induced by Gradient Oxidation for High-Efficiency Magnetization Switching

Orbital angular momentum flow can be used to develop a low-dissipation electronic information device by manipulating the orbital current. However, efficiently generating and fully harnessing orbital currents is a formidable challenge. In this study, an approach is presented that induces a colossal orbital current by gradient oxidation in Pt/Ta to enhance spin-orbit torque (SOT) and achieve high-efficiency magnetization switching. The maximum efficiency of the SOT before and after the gradient oxidation of Ta is improved relative to that of Pt by approximate to 600 and 1200%, respectively. The large SOT originates from the colossal orbital current because of the orbital Rashba-Edelstein effect induced by the gradient oxidation of Ta. In addition, a large spin-to-charge conversion efficiency is observed in yttrium iron garnet/Pt/TaOx because of the inverse orbital Rashba-Edelstein effect. Harnessing the orbital current can help effectively minimize the critical current density of the current-induced magnetization switching to 2.26-1.08 x 106 A cm-2, marking a 12-fold reduction compared to that using Pt. This findings provide a new path for research on low-dissipation spin-orbit devices and improve the tunability of orbital current generation. This study presents an approach involving the enhancement of orbital current generation through gradient oxidation in Pt/Ta for achieving high-efficiency magnetization switching. The significant enhancement of orbital current generation efficiency is attributed to the orbital Rashba-Edelstein effect caused by the symmetry breaking of Pt/TaOx interface inversion. This will provide a new avenue for the research of low-dissipation spintronics devices. image