Composition Characteristics and Potential Regions of PM2.5 during Winter Haze Pollution in Typical Industrial Areas, NW-China

被引:1
作者
Guo, Liyao [1 ]
Gu, Chao [2 ]
Dong, Kaiyuan [3 ]
Ou, Shengju [4 ]
Zhao, Xueyan [1 ]
Wang, Xinhua [1 ]
Zheng, Zhensen [1 ]
Yang, Wen [1 ]
机构
[1] Chinese Res Inst Environm Sci, State Key Lab Environm Criteria & Risk Assessment, Beijing 100012, Peoples R China
[2] Ecol Environm Monitoring Ctr Xinjiang Uygur Autono, Urumqi 830011, Peoples R China
[3] Dept Ecol & Environm Xinjiang Uygur Autonomous Reg, Urumqi 830011, Peoples R China
[4] Nanning Normal Univ, Sch Environm & Life Sci, Naning 530001, Peoples R China
关键词
PM; 2.5; Composition characteristics; Source appointment; Potential sources; TIANJIN-HEBEI REGION; RIVER DELTA REGION; SOURCE APPORTIONMENT; CHEMICAL-CHARACTERIZATION; CARBONACEOUS AEROSOLS; SIZE DISTRIBUTION; AMBIENT PM2.5; MASS CLOSURE; IMPACT; PM10;
D O I
10.4209/aaqr.230290
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
To investigative the causes and potential sources of fine particulate matter (PM2.5) pollution during winter haze pollution in typical industrial areas in northwest China, PM2.5 samples were collected during a winter extreme pollution event (from January 15 to January 29, 2016). The daily average PM2.5 concentrations were -210 mu g m-3 and peak daily concentrations were -496 mu g m-3 in the Kuitun-Dushanzi-Wusu (K-D-W region) of Xinjiang Uygur Autonomous Region, China. Eightyeight samples (including 44 quartz and 44 Teflon samples for PM2.5) were assessed for watersoluble ions (WSIIs), organic/elemental carbon (OC/EC) and inorganic elements. The results showed that the percentage of carbonaceous compounds decreased with more severe pollution levels, and the OC and SOC decreased more rapidly than EC. The sum of 39 inorganic element concentrations (8.28% +/- 3.59%) was lower than that of water-soluble ions (63.26% +/- 8.78%) and carbonaceous compounds (10.95% +/- 3.22%). SO42- is the component with the highest percentage, and the percentage of SO42- increases continuously in severe pollution, indicating that secondary transformation of SO42- was more significant during polluted periods. The increased pollution, combined with high relative humidity (RH) increased the liquid water content (LWC), which in turn promoted heterogeneous reactions. The Positive Matrix Factorization (PMF) analysis shows that secondary particulate matter (47%), coal combustion (19%), fugitive dust (14%), industrial sources (10%) and vehicular emissions (10%) are identified as the major emission sources during winter in the K-D-W region. Potential areas in the K-D-W region are distributed in the southeast direction of the 8th Division.
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页数:16
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