Preparation of double network antibacterial hydrogel modified by hydroxamic acid gelatin/polyacrylamide and high efficiency uranium extraction from seawater

被引:1
作者
Qiang, Taotao [1 ,2 ]
Wang, Yu [1 ,2 ]
Ren, Longfang [1 ,2 ]
Chen, Lu [1 ,2 ]
Li, Yaohui [1 ,2 ]
机构
[1] Shaanxi Univ Sci & Technol, Coll Bioresources Chem & Mat Engn, Xian 710021, Shaanxi, Peoples R China
[2] Shaanxi Univ Sci & Technol, Natl Demonstrat Ctr Expt Light Chem Engn Educ, Xian 710021, Peoples R China
来源
JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING | 2024年 / 12卷 / 05期
基金
中国国家自然科学基金;
关键词
Hydrogel; Adsorption; Uranium extraction from seawater; Hydroxamic acid; MECHANICAL-PROPERTIES; COLOUR REACTION; GRAPHENE OXIDE; ADSORPTION; RECOVERY; IONS;
D O I
10.1016/j.jece.2024.114180
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Uranium extracted from seawater can solve the problem of the shortage of uranium on land and provide potential resources for the nuclear power industry. However, the high salinity and low uranium concentration in seawater, coupled with the presence of competing ions and bacteria, pose significant challenges to this technology. In this study, a hydroxyl oxime acid modified gelatin/polyacrylamide double network (Gel/PAM(DN)-HA) hydrogel developed for efficient uranium extraction from seawater. The adsorption capacity of Gel/PAM(DN)-HA hydrogel for uranium in 15 ppm uranium solution was as high as 397.04 mg-U/g-Ads, with a reuse rate of 78.46 % +/- 5.84 % after 5 cycles of adsorption-desorption. Gel/PAM(DN)-HA was immersed in natural seawater for 24 days to evaluate its adsorption capacity. Gel/PAM(DN)-HA demonstrated an impressive uranium extraction capacity of 4.801 mg<middle dot>g(-1). Antibacterial experiments demonstrated that Gel/PAM(DN)-HA can effectively inhibit the Escherichia coli (E. coli ATCC25922) and Staphylococcus aureus (S. aureus ATCC6538). The results highlight the adsorbent's significant potential for extensive utilization in extracting uranium from seawater.
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页数:9
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