Preparation of double network antibacterial hydrogel modified by hydroxamic acid gelatin/polyacrylamide and high efficiency uranium extraction from seawater

被引:1
作者
Qiang, Taotao [1 ,2 ]
Wang, Yu [1 ,2 ]
Ren, Longfang [1 ,2 ]
Chen, Lu [1 ,2 ]
Li, Yaohui [1 ,2 ]
机构
[1] Shaanxi Univ Sci & Technol, Coll Bioresources Chem & Mat Engn, Xian 710021, Shaanxi, Peoples R China
[2] Shaanxi Univ Sci & Technol, Natl Demonstrat Ctr Expt Light Chem Engn Educ, Xian 710021, Peoples R China
来源
JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING | 2024年 / 12卷 / 05期
基金
中国国家自然科学基金;
关键词
Hydrogel; Adsorption; Uranium extraction from seawater; Hydroxamic acid; MECHANICAL-PROPERTIES; COLOUR REACTION; GRAPHENE OXIDE; ADSORPTION; RECOVERY; IONS;
D O I
10.1016/j.jece.2024.114180
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Uranium extracted from seawater can solve the problem of the shortage of uranium on land and provide potential resources for the nuclear power industry. However, the high salinity and low uranium concentration in seawater, coupled with the presence of competing ions and bacteria, pose significant challenges to this technology. In this study, a hydroxyl oxime acid modified gelatin/polyacrylamide double network (Gel/PAM(DN)-HA) hydrogel developed for efficient uranium extraction from seawater. The adsorption capacity of Gel/PAM(DN)-HA hydrogel for uranium in 15 ppm uranium solution was as high as 397.04 mg-U/g-Ads, with a reuse rate of 78.46 % +/- 5.84 % after 5 cycles of adsorption-desorption. Gel/PAM(DN)-HA was immersed in natural seawater for 24 days to evaluate its adsorption capacity. Gel/PAM(DN)-HA demonstrated an impressive uranium extraction capacity of 4.801 mg<middle dot>g(-1). Antibacterial experiments demonstrated that Gel/PAM(DN)-HA can effectively inhibit the Escherichia coli (E. coli ATCC25922) and Staphylococcus aureus (S. aureus ATCC6538). The results highlight the adsorbent's significant potential for extensive utilization in extracting uranium from seawater.
引用
收藏
页数:9
相关论文
共 42 条
  • [31] Quaternized and Hyperbranched Amidoxime-Modified Ultra-High-Molecular-Weight Polyethylene Fiber for Uranium Extraction from Seawater
    Hu, Lijun
    Han, Hongwei
    Mao, Xuanzhi
    Feng, Xinxin
    He, Yulong
    Hu, Jiangtao
    Wu, Guozhong
    POLYMERS, 2024, 16 (23)
  • [32] Ca/Mg bimetallic MOFs modified with amidoximerized polyacrylonitrile and high efficiency uranium(VI) extraction from solution
    Diao, Shilin
    Li, Mengfang
    Liu, Xuan
    Liu, Yujia
    Shang, Qingjin
    Xu, Yewei
    JOURNAL OF SOLID STATE CHEMISTRY, 2024, 338
  • [33] A high-flux antibacterial poly(amidoxime)-polyacrylonitrile blend membrane for highly efficient uranium extraction from seawater
    Yu, Jiaqi
    Zhang, Hongsen
    Liu, Qi
    Zhu, Jiahui
    Yu, Jing
    Sun, Gaohui
    Li, Rumin
    Wang, Jun
    JOURNAL OF HAZARDOUS MATERIALS, 2022, 440
  • [34] Facile preparation of hydrogel glue with high strength and antibacterial activity from physically linked network
    Yang, Qiao
    Lai, Xinqiao
    Ling, Jiandi
    Chen, Dongque
    Liu, Peng
    Mao, Taoyan
    Shang, Xiaoqin
    Wang, Liming
    INTERNATIONAL JOURNAL OF PHARMACEUTICS, 2022, 622
  • [35] MOF-derived Co-Ni layered double hydroxides/polyethyleneimine modified chitosan micro-nanoreactor for high-efficiency capture of uranium from seawater
    Yu, Jiaqi
    Wang, Jun
    Zhang, Hongsen
    Liu, Qi
    Liu, Jingyuan
    Zhu, Jiahui
    Yu, Jing
    Chen, Rongrong
    CARBOHYDRATE POLYMERS, 2024, 323
  • [36] High-strength ionic hydrogel constructed by metal-free physical crosslinking strategy for enhanced uranium extraction from seawater
    Wang, Yuan-Hao
    Xiang, Yu-Qin
    Huang, Qian
    Yang, Xiao-Lan
    Wang, Shuang-Long
    Zhou, Yue-Ru
    Qin, Song
    Gou, Ling-Qiong
    Tao, Guo-Hong
    He, Ling
    CHEMICAL ENGINEERING JOURNAL, 2024, 479
  • [37] Poly(amidoxime)/polyzwitterionic semi-interpenetrating network hydrogel with robust salt-shrinkage resistance for enhanced uranium extraction from seawater
    Cao, Meng
    Luo, Guangsheng
    Peng, Qin
    Wang, Lushuang
    Wang, Yue
    Zhao, Shilei
    Wang, Hui
    Zhang, Jiacheng
    Yuan, Yihui
    Wang, Ning
    CHEMICAL ENGINEERING JOURNAL, 2024, 481
  • [38] Antibacterial AO-CS/CdS-porous few-layer g-C3N4 nanofiber membrane for high-efficiency uranium extraction from seawater: A dual adsorption-photocatalytic regulation strategy
    Yu, Jiaqi
    Zhang, Hongsen
    Liu, Qi
    Yu, Jing
    Zhu, Jiahui
    Li, Rumin
    Liu, Peili
    Li, Ying
    Wang, Jun
    CHEMICAL ENGINEERING JOURNAL, 2023, 471
  • [39] A high-flux phytic acid functionalized SiO2 blend polysulfone ultrafiltration membrane for extraction of uranium from seawater
    Sun, Haowen
    Liu, Qi
    Liu, Jingyuan
    Zhu, Jiahui
    Yu, Jing
    Chen, Rongrong
    Li, Rumin
    Wang, Jun
    JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING, 2024, 12 (05):
  • [40] Preparation and characterization of hybrid double network chitosan/poly(acrylic amide-acrylic acid) high toughness hydrogel through Al3+ crosslinking
    Jiang, Xiancai
    Xiang, Nanping
    Wang, Jinquan
    Zhao, Yulai
    Hou, Linxi
    CARBOHYDRATE POLYMERS, 2017, 173 : 701 - 706