Micromixing Diffusion Combustion Characteristics of Ammonia Cracking Gas

被引:0
作者
Huang, Hanting [1 ,2 ]
Li, Pengxiang [1 ,2 ]
Xian, Guoli [1 ,2 ]
Mao, Xun [1 ,2 ]
Zhang, Zequn [1 ,2 ]
Wang, Tong [1 ,2 ]
Wang, Jiawei [1 ,2 ]
Wang, Tao [1 ,2 ]
Zhang, Yongsheng [1 ,2 ]
机构
[1] North China Elect Power Univ, Key Lab Condit Monitoring & Control Power Plant Eq, Minist Educ, Beijing 102206, Peoples R China
[2] Beijing Municipal Educ Commiss, Beijing Lab New Energy Storage Technol, Beijing 102206, Peoples R China
关键词
micromixing combustion; ammonia cracking gas; combustion characteristics; NO x; LAMINAR BURNING VELOCITY; TRAPPED VORTEX; FLAME; MIXTURES; TEMPERATURES; EMISSIONS;
D O I
10.1021/acs.energyfuels.4c03055
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
Ammonia cracking combustion can significantly enhance combustion stability, reducing fuel-NOx and ammonia emissions. The combustion characteristics of a micromixing diffusion flame were studied by simulating ammonia cracking gas with ammonia, hydrogen, and nitrogen in this paper. The results indicate that the flame height increases as the cracking ratio decreases and the equivalence ratio increases. Additionally, the flame changes from a yellow color to light blue with insignificant flame height change during increasing cracking ratio. For a 10 kW flame, combustion stability can be maintained when X-cra is above 50%, but there is a risk of flame lifting and blow-off when it is below 40%. When the cracking ratio increases, the nozzle temperature rises. When the equivalence ratio increases, the nozzle temperature reaches a peak and moves with the cracking ratio. As the cracking ratio decreases, the NOx emission increases and then decreases, reaching a maximum value of 910 ppm. The NOx emission is lowest at a cracking ratio of X-cra = 100%, ranging from 2 to 4 ppm. In the case of the lowest cracking ratio (X-cra = 50%), the ammonia in the low-temperature ambient of the combustion chamber plays a significant role in the reduction, resulting in NOx emissions ranging from 44 to 80 ppm. Overall, NOx emission decreases with increasing equivalence ratio, but higher power is accompanied by a greater concentration of NOx emission. Hydrogen near-completely combusts at high cracking ratios. Conversely, decreasing the cracking ratio leads to an increase in ammonia, reduces combustion efficiency, and consequently, results in higher hydrogen emissions, with a peak emission of 28.1 ppm at a 50% cracking ratio and 0.9 equivalence ratio. The results demonstrate that combining ammonia cracking gas with micromixing diffusion combustion can achieve stable and efficient combustion. Low NOx emission can be achieved by controlling influencing factors such as combustion temperature, equivalence ratio, and cracking ratio.
引用
收藏
页码:18988 / 19001
页数:14
相关论文
共 42 条
  • [1] Characteristics of NH3/H2 blend as carbon-free fuels: A review
    Awad, Omar I.
    Zhou, Bo
    Harrath, Karim
    Kadirgama, K.
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2023, 48 (96) : 38077 - 38100
  • [2] Beer J. M., 1972, COMBUSTION AERODYNAM
  • [3] Transitioning from low-emission dry micro-mix hydrogen-air combustion to zero-emission wet micro-mix hydrogen-oxygen combustion in hydrogen energy storage systems
    Boretti, Alberto
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2024, 67 : 1066 - 1073
  • [4] Overview of Autoignition and Flame Propagation Properties for Ammonia Combustion
    Cai, Tao
    Zhao, Dan
    [J]. AIAA JOURNAL, 2023, 61 (07) : 2754 - 2778
  • [5] Overview of fundamental kinetic mechanisms and emission mitigation in ammonia combustion
    Cai, Tao
    Zhao, Dan
    Gutmark, Ephraim
    [J]. CHEMICAL ENGINEERING JOURNAL, 2023, 458
  • [6] Tailoring reduced mechanisms for predicting flame propagation and ignition characteristics in ammonia and ammonia/hydrogen mixtures
    Cai, Tao
    Zhao, Dan
    Chan, Siew Hwa
    Shahsavari, Mohammad
    [J]. ENERGY, 2022, 260
  • [7] Prediction of NOx emissions and pathways in premixed ammonia-hydrogen-air combustion using CFD-CRN methodology
    Chaturvedi, Shivansh
    Santhosh, R.
    Mashruk, Syed
    Yadav, Rajneesh
    Valera-Medina, Agustin
    [J]. JOURNAL OF THE ENERGY INSTITUTE, 2023, 111
  • [8] Effect of hydrogen blending on the high temperature auto-ignition of ammonia at elevated pressure
    Chen, Jundie
    Jiang, Xue
    Qin, Xiaokang
    Huang, Zuohua
    [J]. FUEL, 2021, 287
  • [9] Numerical study of guide vane effects on reacting flow characteristics in a trapped vortex combustor
    Chen, Song
    Zhao, Dan
    [J]. COMBUSTION SCIENCE AND TECHNOLOGY, 2018, 190 (12) : 2111 - 2133
  • [10] Modeling nitrogen chemistry in combustion
    Glarborg, Peter
    Miller, James A.
    Ruscic, Branko
    Klippenstein, Stephen J.
    [J]. PROGRESS IN ENERGY AND COMBUSTION SCIENCE, 2018, 67 : 31 - 68