Analysing the efficacy of TiO2/g-C3N4 nanohybrid electrospun membranes for visible-light photocatalytic water purification

被引:1
|
作者
Padmanabhan, Nisha T. [1 ,2 ,3 ]
Sabin, Christeena [1 ]
Krishnan, H. Unni [1 ]
Hrithik, M. [1 ]
Mythili, Ushamani [2 ,3 ]
Jayaraj, Madambi K. [4 ]
John, Honey [1 ,5 ]
机构
[1] Cochin Univ Sci & Technol, Inter Univ Ctr Nanomat & Devices, Kalamassery 682022, India
[2] St Teresas Coll Autonomous, Dept Phys, Ernakulam 682011, India
[3] St Teresas Coll, Ctr Res, Ernakulam 682011, India
[4] Univ Calicut, Thenhipalam 673635, Kerala, India
[5] Cochin Univ Sci & Technol, Dept Polymer Sci & Rubber Technol, Kochi 682022, India
关键词
Electrospinning technique; Titania; Wettability; Water treatment; Photodegradation; METHYLENE-BLUE; TIO2; HYBRID; DEGRADATION; HETEROJUNCTIONS; PERFORMANCE; EFFICIENCY; G-C3N4; DYE;
D O I
10.1016/j.cplett.2024.141547
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The significance and reliability of membrane-based water purification in wastewater recycling are emphasized in this study. Hydrophilic cellulose acetate and hydrophobic polycaprolactam membranes incorporated with TiO2/ g-C3N4 nanohybrids were fabricated by electrospinning. Synthesis of TiO2/g-C3N4 nanohybrids employed a sol-gel-assisted hydrothermal method, while g-C3N4 through fractional thermal polymerization of acetic acidmodified melamine. The optimized photocatalytic hybrid exhibited methylene blue degradation by a 1.5-fold increase in photoactivity compared to pristine TiO2 and a 3-fold increase compared to g-C3N4. Upon incorporation into electrospun membranes, the hybrids demonstrated effective degradation of Methylene blue dye by photocatalysis, and the membranes exhibited excellent stability over multiple cycles.
引用
收藏
页数:10
相关论文
共 50 条
  • [1] Enhanced visible-light photocatalytic activity of g-C3N4/TiO2 films
    Boonprakob, Natkritta
    Wetchakun, Natda
    Phanichphant, Sukon
    Waxler, David
    Sherrell, Peter
    Nattestad, Andrew
    Chen, Jun
    Inceesungvorn, Burapat
    JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2014, 417 : 402 - 409
  • [2] Mesoporous TiO2/g-C3N4 Microspheres with Enhanced Visible-Light Photocatalytic Activity
    Wei, Hao
    McMaster, William A.
    Tan, Jeannie Z. Y.
    Cao, Lu
    Chen, Dehong
    Caruso, Rachel A.
    JOURNAL OF PHYSICAL CHEMISTRY C, 2017, 121 (40): : 22114 - 22122
  • [4] Synthesis of Porous TiO2/g-C3N4 Nanocomposites with Enhanced Visible-Light Photocatalytic Properties
    Yang Hui
    Shen Jianchao
    Feng Yu
    Cai Qifeng
    Wu Chunchun
    Ma Qingsong
    Shen Qianhong
    RARE METAL MATERIALS AND ENGINEERING, 2016, 45 : 467 - 471
  • [5] Visible-light photocatalytic membranes based on heterostructured Fe3O4-doped g-C3N4/TiO2 catalysts
    Wang, Long
    Zhao, Liu-Lin
    He, Qin-Yuan
    Shao, Dan-Dan
    Sun, Shi-Peng
    Cao, Xue-Li
    JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY, 2023, 98 (09) : 2136 - 2145
  • [6] Effect of TiO2 Morphology on the Properties and Photocatalytic Activity of g-C3N4/TiO2 Nanocomposites Under Visible-Light Illumination
    Roskaric, Matevz
    Zerjav, Gregor
    Zavasnik, Janez
    Finsgar, Matjaz
    Pintar, Albin
    MOLECULES, 2025, 30 (03):
  • [7] Ag–TiO2 mesocrystal-coupled g-C3N4 nanosheets with enhanced visible-light photocatalytic activity
    Fenghua Chen
    Maosen Yang
    Xiangdong Shi
    Xiaoyun Qin
    Qingtao Chen
    Liying Jiang
    Chunxiao Jia
    Research on Chemical Intermediates, 2023, 49 : 101 - 119
  • [8] Construction of g-C3N4/TiO2/Ag composites with enhanced visible-light photocatalytic activity and antibacterial properties
    Yan, Dong
    Wu, Xin
    Pei, Jiayun
    Wu, Chaochao
    Wang, Xiumei
    Zhao, Haiyan
    CERAMICS INTERNATIONAL, 2020, 46 (01) : 696 - 702
  • [9] MOF-derived TiO2 modified with g-C3N4 nanosheets for enhanced visible-light photocatalytic performance
    Li, Ping
    Zhang, Xiaoxian
    Qiu, Lingfang
    Xu, Xun
    Si, Ying
    Liang, Tingting
    Liu, Huan
    Chu, Jingjing
    Guo, Jixin
    Duo, Shuwang
    NEW JOURNAL OF CHEMISTRY, 2020, 44 (17) : 6958 - 6964
  • [10] Growth of MoS2 nanosheets on TiO2/g-C3N4 nanocomposites to enhance the visible-light photocatalytic ability
    Zhang, Rui-Zhi
    Chen, Qi-Wen
    Lei, Yu-Xi
    Zhou, Jian-Ping
    JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2019, 30 (06) : 5393 - 5403