Driven Self-Assembly of Patchy Particles Overcoming Equilibrium Limitations

被引：5

作者：

Nag, Shubhadeep ^{[1
]}

Bisker, Gili ^{[1
]}

机构：

[1] Tel Aviv Univ, Fac Engn, Dept Biomed Engn, IL-6997801 Tel Aviv, Israel

来源：

JOURNAL OF CHEMICAL THEORY AND COMPUTATION | 2024年 / 20卷 / 18期

基金：

欧洲研究理事会;

关键词：

ORGANIZATION; MECHANICS; SYSTEMS;

D O I：

10.1021/acs.jctc.4c01118

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Bridging biological complexity and synthetic material design, we investigate dissipative self-assembly in patchy particle systems. Utilizing Monte Carlo and Molecular Dynamics simulations, we demonstrate how external driving forces mitigate equilibrium trade-offs between assembly time and structural stability, traditionally encountered in self-assembly processes. Our findings also extend to biological-mimicking environments, where we explore the dynamics of patchy particles under crowded conditions. This comprehensive analysis offers insights into advanced material design, opening avenues for innovations in nanotechnology applications.

引用

页码：7700 / 7707

页数：8

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